Articles | Volume 20, issue 5
https://doi.org/10.5194/tc-20-3235-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/tc-20-3235-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Inter-annual snow accumulation and meter-scale variability from trench measurements at Dome C, Antarctica
Adrien Ooms
CORRESPONDING AUTHOR
Laboratoire des Sciences du Climat et de l'Environnement, LSCE/IPSL, CEA-CNRS-UVSQ, Université Paris-Saclay, Gif sur Yvette, France
Mathieu Casado
CORRESPONDING AUTHOR
Laboratoire des Sciences du Climat et de l'Environnement, LSCE/IPSL, CEA-CNRS-UVSQ, Université Paris-Saclay, Gif sur Yvette, France
Ghislain Picard
Institut des Geosciences de l'Environnement (IGE), Université Grenoble Alpes/CNRS, UMR 5001, Grenoble, France
Laurent Arnaud
Institut des Geosciences de l'Environnement (IGE), Université Grenoble Alpes/CNRS, UMR 5001, Grenoble, France
Maria Hörhold
Department of Geosciences, Alfred-Wegener-Institut Helmholtz-Zentrum für Polar- und Meeresforschung, Bremerhaven, Germany
Andrea Spolaor
Institute of Polar Sciences, National Research Council of Italy (ISP-CNR), Venice, Italy
Rita Traversi
Institute of Polar Sciences, National Research Council of Italy (ISP-CNR), Venice, Italy
Joel Savarino
Institut des Geosciences de l'Environnement (IGE), Université Grenoble Alpes/CNRS, UMR 5001, Grenoble, France
Patrick Ginot
Institut des Geosciences de l'Environnement (IGE), Université Grenoble Alpes/CNRS, UMR 5001, Grenoble, France
Pete Akers
Discipline of Geography, School of Natural Sciences, Trinity College Dublin, Dublin, Ireland
Birthe Twarloh
Department of Geosciences, Alfred-Wegener-Institut Helmholtz-Zentrum für Polar- und Meeresforschung, Bremerhaven, Germany
Valérie Masson-Delmotte
Laboratoire des Sciences du Climat et de l'Environnement, LSCE/IPSL, CEA-CNRS-UVSQ, Université Paris-Saclay, Gif sur Yvette, France
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Atmos. Chem. Phys., 25, 16215–16232, https://doi.org/10.5194/acp-25-16215-2025, https://doi.org/10.5194/acp-25-16215-2025, 2025
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Marco Zanatta, Pia Bogert, Patrick Ginot, Yiwei Gong, Gholam Ali Hoshyaripour, Yaqiong Hu, Feng Jiang, Paolo Laj, Yanxia Li, Claudia Linke, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Nsikanabasi Silas Umo, Franziska Vogel, and Robert Wagner
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Agnese Petteni, Elise Fourré, Elsa Gautier, Azzurra Spagnesi, Roxanne Jacob, Pete D. Akers, Daniele Zannoni, Jacopo Gabrieli, Olivier Jossoud, Frédéric Prié, Amaëlle Landais, Titouan Tcheng, Barbara Stenni, Joel Savarino, Patrick Ginot, and Mathieu Casado
Atmos. Meas. Tech., 18, 5435–5455, https://doi.org/10.5194/amt-18-5435-2025, https://doi.org/10.5194/amt-18-5435-2025, 2025
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Amna Ijaz, Brice Temime-Roussel, Benjamin Chazeau, Sarah Albertin, Stephen R. Arnold, Brice Barret, Slimane Bekki, Natalie Brett, Meeta Cesler-Maloney, Elsa Dieudonne, Kayane K. Dingilian, Javier G. Fochesatto, Jingqiu Mao, Allison Moon, Joel Savarino, William Simpson, Rodney J. Weber, Kathy S. Law, and Barbara D'Anna
Atmos. Chem. Phys., 25, 11789–11811, https://doi.org/10.5194/acp-25-11789-2025, https://doi.org/10.5194/acp-25-11789-2025, 2025
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Agnese Petteni, Mathieu Casado, Christophe Leroy-Dos Santos, Amaelle Landais, Niels Dutrievoz, Cécile Agosta, Pete D. Akers, Joel Savarino, Andrea Spolaor, Massimo Frezzotti, and Barbara Stenni
EGUsphere, https://doi.org/10.5194/egusphere-2025-3188, https://doi.org/10.5194/egusphere-2025-3188, 2025
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Lison Soussaintjean, Jochen Schmitt, Joël Savarino, J. Andy Menking, Edward J. Brook, Barbara Seth, Vladimir Lipenkov, Thomas Röckmann, and Hubertus Fischer
EGUsphere, https://doi.org/10.5194/egusphere-2025-3108, https://doi.org/10.5194/egusphere-2025-3108, 2025
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Piers M. Forster, Chris Smith, Tristram Walsh, William F. Lamb, Robin Lamboll, Christophe Cassou, Mathias Hauser, Zeke Hausfather, June-Yi Lee, Matthew D. Palmer, Karina von Schuckmann, Aimée B. A. Slangen, Sophie Szopa, Blair Trewin, Jeongeun Yun, Nathan P. Gillett, Stuart Jenkins, H. Damon Matthews, Krishnan Raghavan, Aurélien Ribes, Joeri Rogelj, Debbie Rosen, Xuebin Zhang, Myles Allen, Lara Aleluia Reis, Robbie M. Andrew, Richard A. Betts, Alex Borger, Jiddu A. Broersma, Samantha N. Burgess, Lijing Cheng, Pierre Friedlingstein, Catia M. Domingues, Marco Gambarini, Thomas Gasser, Johannes Gütschow, Masayoshi Ishii, Christopher Kadow, John Kennedy, Rachel E. Killick, Paul B. Krummel, Aurélien Liné, Didier P. Monselesan, Colin Morice, Jens Mühle, Vaishali Naik, Glen P. Peters, Anna Pirani, Julia Pongratz, Jan C. Minx, Matthew Rigby, Robert Rohde, Abhishek Savita, Sonia I. Seneviratne, Peter Thorne, Christopher Wells, Luke M. Western, Guido R. van der Werf, Susan E. Wijffels, Valérie Masson-Delmotte, and Panmao Zhai
Earth Syst. Sci. Data, 17, 2641–2680, https://doi.org/10.5194/essd-17-2641-2025, https://doi.org/10.5194/essd-17-2641-2025, 2025
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In a rapidly changing climate, evidence-based decision-making benefits from up-to-date and timely information. Here we compile monitoring datasets to track real-world changes over time. To make our work relevant to policymakers, we follow methods from the Intergovernmental Panel on Climate Change (IPCC). Human activities are increasing the Earth's energy imbalance and driving faster sea-level rise compared to the IPCC assessment.
Zhao Wei, Shohei Hattori, Asuka Tsuruta, Zhuang Jiang, Sakiko Ishino, Koji Fujita, Sumito Matoba, Lei Geng, Alexis Lamothe, Ryu Uemura, Naohiro Yoshida, Joel Savarino, and Yoshinori Iizuka
Atmos. Chem. Phys., 25, 5727–5742, https://doi.org/10.5194/acp-25-5727-2025, https://doi.org/10.5194/acp-25-5727-2025, 2025
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Nitrate isotope records in ice cores reveal changes in NOₓ emissions and atmospheric oxidation chemistry driven by human activity. However, UV-driven postdepositional processes can alter nitrate in snow, making snow accumulation rates critical for preserving these records. This study examines nitrate isotopes in a southeastern Greenland ice core, where high snow accumulation minimizes these effects, providing a reliable archive of atmospheric nitrogen cycling.
Florent Domine, Mireille Quémener, Ludovick Bégin, Benjamin Bouchard, Valérie Dionne, Sébastien Jerczynski, Raphaël Larouche, Félix Lévesque-Desrosiers, Simon-Olivier Philibert, Marc-André Vigneault, Ghislain Picard, and Daniel C. Côté
The Cryosphere, 19, 1757–1774, https://doi.org/10.5194/tc-19-1757-2025, https://doi.org/10.5194/tc-19-1757-2025, 2025
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Shrubs buried in snow absorb solar radiation and reduce irradiance in the snowpack. This decreases photochemical reaction rates and emissions to the atmosphere. By monitoring irradiance in snowpacks with and without shrubs, we conclude that shrubs absorb solar radiation as much as 140 ppb of soot and reduce irradiance by a factor of 2. Shrub expansion in the Arctic may therefore affect tropospheric composition during the snow season with climatic effects.
Brice Barret, Patrice Medina, Natalie Brett, Roman Pohorsky, Kathy S. Law, Slimane Bekki, Gilberto J. Fochesatto, Julia Schmale, Steve R. Arnold, Andrea Baccarini, Maurizio Busetto, Meeta Cesler-Maloney, Barbara D'Anna, Stefano Decesari, Jingqiu Mao, Gianluca Pappaccogli, Joel Savarino, Federico Scoto, and William R. Simpson
Atmos. Meas. Tech., 18, 1163–1184, https://doi.org/10.5194/amt-18-1163-2025, https://doi.org/10.5194/amt-18-1163-2025, 2025
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The Fairbanks area experiences severe pollution episodes in winter because of enhanced emissions of pollutants trapped near the surface by strong temperature inversions. Low-cost sensors were deployed on board a car and a tethered balloon to measure the concentrations of gaseous pollutants (CO, O3, and NOx) in Fairbanks during winter 2022. Data calibration with reference measurements and machine learning methods enabled us to document pollution at the surface and power plant plumes aloft.
Rémi Dallmayr, Hannah Meyer, Vasileios Gkinis, Thomas Laepple, Melanie Behrens, Frank Wilhelms, and Maria Hörhold
The Cryosphere, 19, 1067–1083, https://doi.org/10.5194/tc-19-1067-2025, https://doi.org/10.5194/tc-19-1067-2025, 2025
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Recent studies showed that a large number of independent vertical profiles allow for inferring a common local climate signal from the stacked stable water isotope record. Through investigating instrumental limitation and the effect of percolation of such porous samples, this study assesses the continuous flow analysis (CFA) technique in order to analyze the significant number of snow surface profiles within a reasonable time and with high quality.
Thomas Lauwers, Elise Fourré, Olivier Jossoud, Daniele Romanini, Frédéric Prié, Giordano Nitti, Mathieu Casado, Kévin Jaulin, Markus Miltner, Morgane Farradèche, Valérie Masson-Delmotte, and Amaëlle Landais
Atmos. Meas. Tech., 18, 1135–1147, https://doi.org/10.5194/amt-18-1135-2025, https://doi.org/10.5194/amt-18-1135-2025, 2025
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Water vapour isotopes are important tools to better understand processes governing the atmospheric hydrological cycle. In polar regions, their measurement helps to improve the interpretation of water isotopic records in ice cores. However, in situ water vapour isotopic monitoring is an important challenge, especially in dry places of East Antarctica. We present here an alternative laser spectroscopy technique adapted for such measurements, with a limit of detection down to 10 ppm humidity.
Natalie Brett, Kathy S. Law, Steve R. Arnold, Javier G. Fochesatto, Jean-Christophe Raut, Tatsuo Onishi, Robert Gilliam, Kathleen Fahey, Deanna Huff, George Pouliot, Brice Barret, Elsa Dieudonné, Roman Pohorsky, Julia Schmale, Andrea Baccarini, Slimane Bekki, Gianluca Pappaccogli, Federico Scoto, Stefano Decesari, Antonio Donateo, Meeta Cesler-Maloney, William Simpson, Patrice Medina, Barbara D'Anna, Brice Temime-Roussel, Joel Savarino, Sarah Albertin, Jingqiu Mao, Becky Alexander, Allison Moon, Peter F. DeCarlo, Vanessa Selimovic, Robert Yokelson, and Ellis S. Robinson
Atmos. Chem. Phys., 25, 1063–1104, https://doi.org/10.5194/acp-25-1063-2025, https://doi.org/10.5194/acp-25-1063-2025, 2025
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Processes influencing dispersion of local anthropogenic pollution in Arctic wintertime are investigated with Lagrangian dispersion modelling. Simulated power plant plume rise that considers temperature inversion layers improves results compared to observations (interior Alaska). Modelled surface concentrations are improved by representation of vertical mixing and emission estimates. Large increases in diesel vehicle emissions at temperatures reaching −35°C are required to reproduce observed NOx.
Inès Ollivier, Hans Christian Steen-Larsen, Barbara Stenni, Laurent Arnaud, Mathieu Casado, Alexandre Cauquoin, Giuliano Dreossi, Christophe Genthon, Bénédicte Minster, Ghislain Picard, Martin Werner, and Amaëlle Landais
The Cryosphere, 19, 173–200, https://doi.org/10.5194/tc-19-173-2025, https://doi.org/10.5194/tc-19-173-2025, 2025
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The role of post-depositional processes taking place at the ice sheet's surface on the water stable isotope signal measured in polar ice cores is not fully understood. Using field observations and modelling results, we show that the original precipitation isotopic signal at Dome C, East Antarctica, is modified by post-depositional processes and provide the first quantitative estimation of their mean impact on the isotopic signal observed in the snow.
Ghislain Picard and Quentin Libois
Geosci. Model Dev., 17, 8927–8953, https://doi.org/10.5194/gmd-17-8927-2024, https://doi.org/10.5194/gmd-17-8927-2024, 2024
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The Two-streAm Radiative TransfEr in Snow (TARTES) is a radiative transfer model to compute snow albedo in the solar domain and the profiles of light and energy absorption in a multi-layered snowpack whose physical properties are user defined. It uniquely considers snow grain shape flexibly, based on recent insights showing that snow does not behave as a collection of ice spheres but instead as a random medium. TARTES is user-friendly yet performs comparably to more complex models.
Darrell Kaufman and Valérie Masson-Delmotte
Clim. Past, 20, 2587–2594, https://doi.org/10.5194/cp-20-2587-2024, https://doi.org/10.5194/cp-20-2587-2024, 2024
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Rather than reverting to a dedicated paleoclimate chapter, knowledge about pre-industrial climate should be further integrated with other lines of evidence throughout the next assessment reports by the Intergovernmental Panel on Climate Change.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
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Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Luca Teruzzi, Andrea Spolaor, David Cappelletti, Claudio Artoni, and Marco A. C. Potenza
EGUsphere, https://doi.org/10.5194/egusphere-2024-2057, https://doi.org/10.5194/egusphere-2024-2057, 2024
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We present a novel probe to measure visible light penetration into the uppermost snow layers with high spatial resolution. The probe is designed to be lightweight and robust to be exploited in extreme environments, extrapolating to the UV region. Such experimental approach will allow to fill the gap in the current understanding of sunlight propagation through the snowpack, often based on numerical approaches, improving the understanding of those processes occurring in snow even in the UV region.
Melody Sandells, Nick Rutter, Kirsty Wivell, Richard Essery, Stuart Fox, Chawn Harlow, Ghislain Picard, Alexandre Roy, Alain Royer, and Peter Toose
The Cryosphere, 18, 3971–3990, https://doi.org/10.5194/tc-18-3971-2024, https://doi.org/10.5194/tc-18-3971-2024, 2024
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Satellite microwave observations are used for weather forecasting. In Arctic regions this is complicated by natural emission from snow. By simulating airborne observations from in situ measurements of snow, this study shows how snow properties affect the signal within the atmosphere. Fresh snowfall between flights changed airborne measurements. Good knowledge of snow layering and structure can be used to account for the effects of snow and could unlock these data to improve forecasts.
Giuliano Dreossi, Mauro Masiol, Barbara Stenni, Daniele Zannoni, Claudio Scarchilli, Virginia Ciardini, Mathieu Casado, Amaëlle Landais, Martin Werner, Alexandre Cauquoin, Giampietro Casasanta, Massimo Del Guasta, Vittoria Posocco, and Carlo Barbante
The Cryosphere, 18, 3911–3931, https://doi.org/10.5194/tc-18-3911-2024, https://doi.org/10.5194/tc-18-3911-2024, 2024
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Oxygen and hydrogen stable isotopes have been extensively used to reconstruct past temperatures, with precipitation representing the input signal of the isotopic records in ice cores. We present a 10-year record of stable isotopes in daily precipitation at Concordia Station: this is the longest record for inland Antarctica and represents a benchmark for quantifying post-depositional processes and improving the paleoclimate interpretation of ice cores.
Sara Arioli, Ghislain Picard, Laurent Arnaud, Simon Gascoin, Esteban Alonso-González, Marine Poizat, and Mark Irvine
Earth Syst. Sci. Data, 16, 3913–3934, https://doi.org/10.5194/essd-16-3913-2024, https://doi.org/10.5194/essd-16-3913-2024, 2024
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High-accuracy precision maps of the surface temperature of snow were acquired with an uncooled thermal-infrared camera during winter 2021–2022 and spring 2023. The accuracy – i.e., mean absolute error – improved from 1.28 K to 0.67 K between the seasons thanks to an improved camera setup and temperature stabilization. The dataset represents a major advance in the validation of satellite measurements and physical snow models over a complex topography.
Romilly Harris Stuart, Amaëlle Landais, Laurent Arnaud, Christo Buizert, Emilie Capron, Marie Dumont, Quentin Libois, Robert Mulvaney, Anaïs Orsi, Ghislain Picard, Frédéric Prié, Jeffrey Severinghaus, Barbara Stenni, and Patricia Martinerie
The Cryosphere, 18, 3741–3763, https://doi.org/10.5194/tc-18-3741-2024, https://doi.org/10.5194/tc-18-3741-2024, 2024
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Ice core δO2/N2 records are useful dating tools due to their local insolation pacing. A precise understanding of the physical mechanism driving this relationship, however, remain ambiguous. By compiling data from 15 polar sites, we find a strong dependence of mean δO2/N2 on accumulation rate and temperature in addition to the well-documented insolation dependence. Snowpack modelling is used to investigate which physical properties drive the mechanistic dependence on these local parameters.
Mathieu Casado, Amaelle Landais, Tim Stoltmann, Justin Chaillot, Mathieu Daëron, Fréderic Prié, Baptiste Bordet, and Samir Kassi
Atmos. Meas. Tech., 17, 4599–4612, https://doi.org/10.5194/amt-17-4599-2024, https://doi.org/10.5194/amt-17-4599-2024, 2024
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Measuring water isotopic composition in Antarctica is difficult because of the extremely cold temperature in winter. Here, we designed a new infrared spectrometer able to measure the vapour isotopic composition during more than 95 % of the year in the coldest locations of Antarctica, whereas current commercial instruments are only able to measure during the warm summer months in the interior.
Piers M. Forster, Chris Smith, Tristram Walsh, William F. Lamb, Robin Lamboll, Bradley Hall, Mathias Hauser, Aurélien Ribes, Debbie Rosen, Nathan P. Gillett, Matthew D. Palmer, Joeri Rogelj, Karina von Schuckmann, Blair Trewin, Myles Allen, Robbie Andrew, Richard A. Betts, Alex Borger, Tim Boyer, Jiddu A. Broersma, Carlo Buontempo, Samantha Burgess, Chiara Cagnazzo, Lijing Cheng, Pierre Friedlingstein, Andrew Gettelman, Johannes Gütschow, Masayoshi Ishii, Stuart Jenkins, Xin Lan, Colin Morice, Jens Mühle, Christopher Kadow, John Kennedy, Rachel E. Killick, Paul B. Krummel, Jan C. Minx, Gunnar Myhre, Vaishali Naik, Glen P. Peters, Anna Pirani, Julia Pongratz, Carl-Friedrich Schleussner, Sonia I. Seneviratne, Sophie Szopa, Peter Thorne, Mahesh V. M. Kovilakam, Elisa Majamäki, Jukka-Pekka Jalkanen, Margreet van Marle, Rachel M. Hoesly, Robert Rohde, Dominik Schumacher, Guido van der Werf, Russell Vose, Kirsten Zickfeld, Xuebin Zhang, Valérie Masson-Delmotte, and Panmao Zhai
Earth Syst. Sci. Data, 16, 2625–2658, https://doi.org/10.5194/essd-16-2625-2024, https://doi.org/10.5194/essd-16-2625-2024, 2024
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This paper tracks some key indicators of global warming through time, from 1850 through to the end of 2023. It is designed to give an authoritative estimate of global warming to date and its causes. We find that in 2023, global warming reached 1.3 °C and is increasing at over 0.2 °C per decade. This is caused by all-time-high greenhouse gas emissions.
Julien Meloche, Melody Sandells, Henning Löwe, Nick Rutter, Richard Essery, Ghislain Picard, Randall K. Scharien, Alexandre Langlois, Matthias Jaggi, Josh King, Peter Toose, Jérôme Bouffard, Alessandro Di Bella, and Michele Scagliola
EGUsphere, https://doi.org/10.5194/egusphere-2024-1583, https://doi.org/10.5194/egusphere-2024-1583, 2024
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Sea ice thickness is essential for climate studies. Radar altimetry has provided sea ice thickness measurement, but uncertainty arises from interaction of the signal with the snow cover. Therefore, modelling the signal interaction with the snow is necessary to improve retrieval. A radar model was used to simulate the radar signal from the snow-covered sea ice. This work paved the way to improved physical algorithm to retrieve snow depth and sea ice thickness for radar altimeter missions.
V. Holly L. Winton, Robert Mulvaney, Joel Savarino, Kyle R. Clem, and Markus M. Frey
Clim. Past, 20, 1213–1232, https://doi.org/10.5194/cp-20-1213-2024, https://doi.org/10.5194/cp-20-1213-2024, 2024
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In 2018, a new 120 m ice core was drilled in a region located under the Antarctic ozone hole. We present the first results including a 1300-year record of snow accumulation and aerosol chemistry. We investigate the aerosol and moisture source regions and atmospheric processes related to the ice core record and discuss what this means for developing a record of past ultraviolet radiation and ozone depletion using the stable isotopic composition of nitrate measured in the same ice core.
Zhuang Jiang, Becky Alexander, Joel Savarino, and Lei Geng
Atmos. Chem. Phys., 24, 4895–4914, https://doi.org/10.5194/acp-24-4895-2024, https://doi.org/10.5194/acp-24-4895-2024, 2024
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Ice-core nitrate could track the past atmospheric NOx and oxidant level, but its interpretation is hampered by the post-depositional processing. In this work, an inverse model was developed and tested against two polar sites and was shown to well reproduce the observed nitrate signals in snow and atmosphere, suggesting that the model can properly correct for the effect of post-depositional processing. This model offers a very useful tool for future studies on ice-core nitrate records.
Tessa R. Vance, Nerilie J. Abram, Alison S. Criscitiello, Camilla K. Crockart, Aylin DeCampo, Vincent Favier, Vasileios Gkinis, Margaret Harlan, Sarah L. Jackson, Helle A. Kjær, Chelsea A. Long, Meredith K. Nation, Christopher T. Plummer, Delia Segato, Andrea Spolaor, and Paul T. Vallelonga
Clim. Past, 20, 969–990, https://doi.org/10.5194/cp-20-969-2024, https://doi.org/10.5194/cp-20-969-2024, 2024
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This study presents the chronologies from the new Mount Brown South ice cores from East Antarctica, which were developed by counting annual layers in the ice core data and aligning these to volcanic sulfate signatures. The uncertainty in the dating is quantified, and we discuss initial results from seasonal cycle analysis and mean annual concentrations. The chronologies will underpin the development of new proxy records for East Antarctica spanning the past millennium.
Amaelle Landais, Cécile Agosta, Françoise Vimeux, Olivier Magand, Cyrielle Solis, Alexandre Cauquoin, Niels Dutrievoz, Camille Risi, Christophe Leroy-Dos Santos, Elise Fourré, Olivier Cattani, Olivier Jossoud, Bénédicte Minster, Frédéric Prié, Mathieu Casado, Aurélien Dommergue, Yann Bertrand, and Martin Werner
Atmos. Chem. Phys., 24, 4611–4634, https://doi.org/10.5194/acp-24-4611-2024, https://doi.org/10.5194/acp-24-4611-2024, 2024
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We have monitored water vapor isotopes since January 2020 on Amsterdam Island in the Indian Ocean. We show 11 periods associated with abrupt negative excursions of water vapor δ18Ο. Six of these events show a decrease in gaseous elemental mercury, suggesting subsidence of air from a higher altitude. Accurately representing the water isotopic signal during these cold fronts is a real challenge for the atmospheric components of Earth system models equipped with water isotopes.
Alexandra M. Zuhr, Sonja Wahl, Hans Christian Steen-Larsen, Maria Hörhold, Hanno Meyer, Vasileios Gkinis, and Thomas Laepple
Earth Syst. Sci. Data, 16, 1861–1874, https://doi.org/10.5194/essd-16-1861-2024, https://doi.org/10.5194/essd-16-1861-2024, 2024
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We present stable water isotope data from the accumulation zone of the Greenland ice sheet. A spatial sampling scheme covering 39 m and three depth layers was carried out between 14 May and 3 August 2018. The data suggest spatial and temporal variability related to meteorological conditions, such as wind-driven snow redistribution and vapour–snow exchange processes. The data can be used to study the formation of the stable water isotopes signal, which is seen as a climate proxy.
Naomi E. Ochwat, Ted A. Scambos, Alison F. Banwell, Robert S. Anderson, Michelle L. Maclennan, Ghislain Picard, Julia A. Shates, Sebastian Marinsek, Liliana Margonari, Martin Truffer, and Erin C. Pettit
The Cryosphere, 18, 1709–1731, https://doi.org/10.5194/tc-18-1709-2024, https://doi.org/10.5194/tc-18-1709-2024, 2024
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On the Antarctic Peninsula, there is a small bay that had sea ice fastened to the shoreline (
fast ice) for over a decade. The fast ice stabilized the glaciers that fed into the ocean. In January 2022, the fast ice broke away. Using satellite data we found that this was because of low sea ice concentrations and a high long-period ocean wave swell. We find that the glaciers have responded to this event by thinning, speeding up, and retreating by breaking off lots of icebergs at remarkable rates.
C. Isabel Moreno, Radovan Krejci, Jean-Luc Jaffrezo, Gaëlle Uzu, Andrés Alastuey, Marcos F. Andrade, Valeria Mardóñez, Alkuin Maximilian Koenig, Diego Aliaga, Claudia Mohr, Laura Ticona, Fernando Velarde, Luis Blacutt, Ricardo Forno, David N. Whiteman, Alfred Wiedensohler, Patrick Ginot, and Paolo Laj
Atmos. Chem. Phys., 24, 2837–2860, https://doi.org/10.5194/acp-24-2837-2024, https://doi.org/10.5194/acp-24-2837-2024, 2024
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Aerosol chemical composition (ions, sugars, carbonaceous matter) from 2011 to 2020 was studied at Mt. Chacaltaya (5380 m a.s.l., Bolivian Andes). Minimum concentrations occur in the rainy season with maxima in the dry and transition seasons. The origins of the aerosol are located in a radius of hundreds of kilometers: nearby urban and rural areas, natural biogenic emissions, vegetation burning from Amazonia and Chaco, Pacific Ocean emissions, soil dust, and Peruvian volcanism.
Justin Murfitt, Claude Duguay, Ghislain Picard, and Juha Lemmetyinen
The Cryosphere, 18, 869–888, https://doi.org/10.5194/tc-18-869-2024, https://doi.org/10.5194/tc-18-869-2024, 2024
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This research focuses on the interaction between microwave signals and lake ice under wet conditions. Field data collected for Lake Oulujärvi in Finland were used to model backscatter under different conditions. The results of the modelling likely indicate that a combination of increased water content and roughness of different interfaces caused backscatter to increase. These results could help to identify areas where lake ice is unsafe for winter transportation.
Claudio Stefanini, Giovanni Macelloni, Marion Leduc-Leballeur, Vincent Favier, Benjamin Pohl, and Ghislain Picard
The Cryosphere, 18, 593–608, https://doi.org/10.5194/tc-18-593-2024, https://doi.org/10.5194/tc-18-593-2024, 2024
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Local and large-scale meteorological conditions have been considered in order to explain some peculiar changes of snow grains on the East Antarctic Plateau from 2000 to 2022, by using remote sensing observations and reanalysis. We identified some extreme grain size events on the highest ice divide, resulting from a combination of conditions of low wind speed and low temperature. Moreover, the beginning of seasonal grain growth has been linked to the occurrence of atmospheric rivers.
Sarah Albertin, Joël Savarino, Slimane Bekki, Albane Barbero, Roberto Grilli, Quentin Fournier, Irène Ventrillard, Nicolas Caillon, and Kathy Law
Atmos. Chem. Phys., 24, 1361–1388, https://doi.org/10.5194/acp-24-1361-2024, https://doi.org/10.5194/acp-24-1361-2024, 2024
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This study reports the first simultaneous records of oxygen (Δ17O) and nitrogen (δ15N) isotopes in nitrogen dioxide (NO2) and nitrate (NO3−). These data are combined with atmospheric observations to explore sub-daily N reactive chemistry and quantify N fractionation effects in an Alpine winter city. The results highlight the necessity of using Δ17O and δ15N in both NO2 and NO3− to avoid biased estimations of NOx sources and fates from NO3− isotopic records in urban winter environments.
Andrea Spolaor, Federico Scoto, Catherine Larose, Elena Barbaro, Francois Burgay, Mats P. Bjorkman, David Cappelletti, Federico Dallo, Fabrizio de Blasi, Dmitry Divine, Giuliano Dreossi, Jacopo Gabrieli, Elisabeth Isaksson, Jack Kohler, Tonu Martma, Louise S. Schmidt, Thomas V. Schuler, Barbara Stenni, Clara Turetta, Bartłomiej Luks, Mathieu Casado, and Jean-Charles Gallet
The Cryosphere, 18, 307–320, https://doi.org/10.5194/tc-18-307-2024, https://doi.org/10.5194/tc-18-307-2024, 2024
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We evaluate the impact of the increased snowmelt on the preservation of the oxygen isotope (δ18O) signal in firn records recovered from the top of the Holtedahlfonna ice field located in the Svalbard archipelago. Thanks to a multidisciplinary approach we demonstrate a progressive deterioration of the isotope signal in the firn core. We link the degradation of the δ18O signal to the increased occurrence and intensity of melt events associated with the rapid warming occurring in the archipelago.
Christophe Leroy-Dos Santos, Elise Fourré, Cécile Agosta, Mathieu Casado, Alexandre Cauquoin, Martin Werner, Benedicte Minster, Frédéric Prié, Olivier Jossoud, Leila Petit, and Amaëlle Landais
The Cryosphere, 17, 5241–5254, https://doi.org/10.5194/tc-17-5241-2023, https://doi.org/10.5194/tc-17-5241-2023, 2023
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In the face of global warming, understanding the changing water cycle and temperatures in polar regions is crucial. These factors directly impact the balance of ice sheets in the Arctic and Antarctic. By studying the composition of water vapor, we gain insights into climate variations. Our 2-year study at Dumont d’Urville station, Adélie Land, offers valuable data to refine models. Additionally, we demonstrate how modeling aids in interpreting signals from ice core samples in the region.
Jean Emmanuel Sicart, Victor Ramseyer, Ghislain Picard, Laurent Arnaud, Catherine Coulaud, Guilhem Freche, Damien Soubeyrand, Yves Lejeune, Marie Dumont, Isabelle Gouttevin, Erwan Le Gac, Frédéric Berger, Jean-Matthieu Monnet, Laurent Borgniet, Éric Mermin, Nick Rutter, Clare Webster, and Richard Essery
Earth Syst. Sci. Data, 15, 5121–5133, https://doi.org/10.5194/essd-15-5121-2023, https://doi.org/10.5194/essd-15-5121-2023, 2023
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Forests strongly modify the accumulation, metamorphism and melting of snow in midlatitude and high-latitude regions. Two field campaigns during the winters 2016–17 and 2017–18 were conducted in a coniferous forest in the French Alps to study interactions between snow and vegetation. This paper presents the field site, instrumentation and collection methods. The observations include forest characteristics, meteorology, snow cover and snow interception by the canopy during precipitation events.
Chiara I. Paleari, Florian Mekhaldi, Tobias Erhardt, Minjie Zheng, Marcus Christl, Florian Adolphi, Maria Hörhold, and Raimund Muscheler
Clim. Past, 19, 2409–2422, https://doi.org/10.5194/cp-19-2409-2023, https://doi.org/10.5194/cp-19-2409-2023, 2023
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In this study, we test the use of excess meltwater from continuous flow analysis from a firn core from Greenland for the measurement of 10Be for solar activity reconstructions. We show that the quality of results is similar to the measurements on clean firn, which opens the possibility to obtain continuous 10Be records without requiring large amounts of clean ice. Furthermore, we investigate the possibility of identifying solar storm signals in 10Be records from Greenland and Antarctica.
Barbara Harm-Altstädter, Konrad Bärfuss, Lutz Bretschneider, Martin Schön, Jens Bange, Ralf Käthner, Radovan Krejci, Mauro Mazzola, Kihong Park, Falk Pätzold, Alexander Peuker, Rita Traversi, Birgit Wehner, and Astrid Lampert
Aerosol Research, 1, 39–64, https://doi.org/10.5194/ar-1-39-2023, https://doi.org/10.5194/ar-1-39-2023, 2023
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We present observations of aerosol particles and meteorological parameters in the horizontal and vertical distribution measured with uncrewed aerial systems in the Arctic. The field campaign was carried out during the snow melting season, when ultrafine aerosol particles (UFPs) with a size between 3 and 12 nm occurred frequently. A high variability of the measured UFPs was identified in the spatial scale, which was strongly associated with different atmospheric boundary layer properties.
Tobias Erhardt, Camilla Marie Jensen, Florian Adolphi, Helle Astrid Kjær, Remi Dallmayr, Birthe Twarloh, Melanie Behrens, Motohiro Hirabayashi, Kaori Fukuda, Jun Ogata, François Burgay, Federico Scoto, Ilaria Crotti, Azzurra Spagnesi, Niccoló Maffezzoli, Delia Segato, Chiara Paleari, Florian Mekhaldi, Raimund Muscheler, Sophie Darfeuil, and Hubertus Fischer
Earth Syst. Sci. Data, 15, 5079–5091, https://doi.org/10.5194/essd-15-5079-2023, https://doi.org/10.5194/essd-15-5079-2023, 2023
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The presented paper provides a 3.8 kyr long dataset of aerosol concentrations from the East Greenland Ice coring Project (EGRIP) ice core. The data consists of 1 mm depth-resolution profiles of calcium, sodium, ammonium, nitrate, and electrolytic conductivity as well as decadal averages of these profiles. Alongside the data a detailed description of the measurement setup as well as a discussion of the uncertainties are given.
Thomas Dethinne, Quentin Glaude, Ghislain Picard, Christoph Kittel, Patrick Alexander, Anne Orban, and Xavier Fettweis
The Cryosphere, 17, 4267–4288, https://doi.org/10.5194/tc-17-4267-2023, https://doi.org/10.5194/tc-17-4267-2023, 2023
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We investigate the sensitivity of the regional climate model
Modèle Atmosphérique Régional(MAR) to the assimilation of wet-snow occurrence estimated by remote sensing datasets. The assimilation is performed by nudging the MAR snowpack temperature. The data assimilation is performed over the Antarctic Peninsula for the 2019–2021 period. The results show an increase in the melt production (+66.7 %) and a decrease in surface mass balance (−4.5 %) of the model for the 2019–2020 melt season.
Nora Hirsch, Alexandra Zuhr, Thomas Münch, Maria Hörhold, Johannes Freitag, Remi Dallmayr, and Thomas Laepple
The Cryosphere, 17, 4207–4221, https://doi.org/10.5194/tc-17-4207-2023, https://doi.org/10.5194/tc-17-4207-2023, 2023
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Stable water isotopes from firn cores provide valuable information on past climates, yet their utility is hampered by stratigraphic noise, i.e. the irregular deposition and wind-driven redistribution of snow. We found stratigraphic noise on the Antarctic Plateau to be related to the local accumulation rate, snow surface roughness and slope inclination, which can guide future decisions on sampling locations and thus increase the resolution of climate reconstructions from low-accumulation areas.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Valeria Mardoñez, Marco Pandolfi, Lucille Joanna S. Borlaza, Jean-Luc Jaffrezo, Andrés Alastuey, Jean-Luc Besombes, Isabel Moreno R., Noemi Perez, Griša Močnik, Patrick Ginot, Radovan Krejci, Vladislav Chrastny, Alfred Wiedensohler, Paolo Laj, Marcos Andrade, and Gaëlle Uzu
Atmos. Chem. Phys., 23, 10325–10347, https://doi.org/10.5194/acp-23-10325-2023, https://doi.org/10.5194/acp-23-10325-2023, 2023
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La Paz and El Alto are two fast-growing, high-altitude Bolivian cities forming the second-largest metropolitan area in the country. The sources of particulate matter (PM) in this conurbation were not previously investigated. This study identified 11 main sources of PM, of which dust and vehicular emissions stand out as the main ones. The influence of regional biomass combustion and local waste combustion was also observed, with the latter being a major source of hazardous compounds.
Alexis Lamothe, Joel Savarino, Patrick Ginot, Lison Soussaintjean, Elsa Gautier, Pete D. Akers, Nicolas Caillon, and Joseph Erbland
Atmos. Meas. Tech., 16, 4015–4030, https://doi.org/10.5194/amt-16-4015-2023, https://doi.org/10.5194/amt-16-4015-2023, 2023
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Ammonia is a reactive gas in our atmosphere that is key in air quality issues. Assessing its emissions and how it reacts is a hot topic that can be addressed from the past. Stable isotopes (the mass of the molecule) measured in ice cores (glacial archives) can teach us a lot. However, the concentrations in ice cores are very small. We propose a protocol to limit the contamination and apply it to one ice core drilled in Mont Blanc, describing the opportunities our method brings.
Yaowen Zheng, Nicholas R. Golledge, Alexandra Gossart, Ghislain Picard, and Marion Leduc-Leballeur
The Cryosphere, 17, 3667–3694, https://doi.org/10.5194/tc-17-3667-2023, https://doi.org/10.5194/tc-17-3667-2023, 2023
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Positive degree-day (PDD) schemes are widely used in many Antarctic numerical ice sheet models. However, the PDD approach has not been systematically explored for its application in Antarctica. We have constructed a novel grid-cell-level spatially distributed PDD (dist-PDD) model and assessed its accuracy. We suggest that an appropriately parameterized dist-PDD model can be a valuable tool for exploring Antarctic surface melt beyond the satellite era.
Esteban Alonso-González, Simon Gascoin, Sara Arioli, and Ghislain Picard
The Cryosphere, 17, 3329–3342, https://doi.org/10.5194/tc-17-3329-2023, https://doi.org/10.5194/tc-17-3329-2023, 2023
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Data assimilation techniques are a promising approach to improve snowpack simulations in remote areas that are difficult to monitor. This paper studies the ability of satellite-observed land surface temperature to improve snowpack simulations through data assimilation. We show that it is possible to improve snowpack simulations, but the temporal resolution of the observations and the algorithm used are critical to obtain satisfactory results.
Marie Dumont, Simon Gascoin, Marion Réveillet, Didier Voisin, François Tuzet, Laurent Arnaud, Mylène Bonnefoy, Montse Bacardit Peñarroya, Carlo Carmagnola, Alexandre Deguine, Aurélie Diacre, Lukas Dürr, Olivier Evrard, Firmin Fontaine, Amaury Frankl, Mathieu Fructus, Laure Gandois, Isabelle Gouttevin, Abdelfateh Gherab, Pascal Hagenmuller, Sophia Hansson, Hervé Herbin, Béatrice Josse, Bruno Jourdain, Irene Lefevre, Gaël Le Roux, Quentin Libois, Lucie Liger, Samuel Morin, Denis Petitprez, Alvaro Robledano, Martin Schneebeli, Pascal Salze, Delphine Six, Emmanuel Thibert, Jürg Trachsel, Matthieu Vernay, Léo Viallon-Galinier, and Céline Voiron
Earth Syst. Sci. Data, 15, 3075–3094, https://doi.org/10.5194/essd-15-3075-2023, https://doi.org/10.5194/essd-15-3075-2023, 2023
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Saharan dust outbreaks have profound effects on ecosystems, climate, health, and the cryosphere, but the spatial deposition pattern of Saharan dust is poorly known. Following the extreme dust deposition event of February 2021 across Europe, a citizen science campaign was launched to sample dust on snow over the Pyrenees and the European Alps. This campaign triggered wide interest and over 100 samples. The samples revealed the high variability of the dust properties within a single event.
Elizabeth R. Thomas, Diana O. Vladimirova, Dieter R. Tetzner, B. Daniel Emanuelsson, Nathan Chellman, Daniel A. Dixon, Hugues Goosse, Mackenzie M. Grieman, Amy C. F. King, Michael Sigl, Danielle G. Udy, Tessa R. Vance, Dominic A. Winski, V. Holly L. Winton, Nancy A. N. Bertler, Akira Hori, Chavarukonam M. Laluraj, Joseph R. McConnell, Yuko Motizuki, Kazuya Takahashi, Hideaki Motoyama, Yoichi Nakai, Franciéle Schwanck, Jefferson Cardia Simões, Filipe Gaudie Ley Lindau, Mirko Severi, Rita Traversi, Sarah Wauthy, Cunde Xiao, Jiao Yang, Ellen Mosely-Thompson, Tamara V. Khodzher, Ludmila P. Golobokova, and Alexey A. Ekaykin
Earth Syst. Sci. Data, 15, 2517–2532, https://doi.org/10.5194/essd-15-2517-2023, https://doi.org/10.5194/essd-15-2517-2023, 2023
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The concentration of sodium and sulfate measured in Antarctic ice cores is related to changes in both sea ice and winds. Here we have compiled a database of sodium and sulfate records from 105 ice core sites in Antarctica. The records span all, or part, of the past 2000 years. The records will improve our understanding of how winds and sea ice have changed in the past and how they have influenced the climate of Antarctica over the past 2000 years.
Piers M. Forster, Christopher J. Smith, Tristram Walsh, William F. Lamb, Robin Lamboll, Mathias Hauser, Aurélien Ribes, Debbie Rosen, Nathan Gillett, Matthew D. Palmer, Joeri Rogelj, Karina von Schuckmann, Sonia I. Seneviratne, Blair Trewin, Xuebin Zhang, Myles Allen, Robbie Andrew, Arlene Birt, Alex Borger, Tim Boyer, Jiddu A. Broersma, Lijing Cheng, Frank Dentener, Pierre Friedlingstein, José M. Gutiérrez, Johannes Gütschow, Bradley Hall, Masayoshi Ishii, Stuart Jenkins, Xin Lan, June-Yi Lee, Colin Morice, Christopher Kadow, John Kennedy, Rachel Killick, Jan C. Minx, Vaishali Naik, Glen P. Peters, Anna Pirani, Julia Pongratz, Carl-Friedrich Schleussner, Sophie Szopa, Peter Thorne, Robert Rohde, Maisa Rojas Corradi, Dominik Schumacher, Russell Vose, Kirsten Zickfeld, Valérie Masson-Delmotte, and Panmao Zhai
Earth Syst. Sci. Data, 15, 2295–2327, https://doi.org/10.5194/essd-15-2295-2023, https://doi.org/10.5194/essd-15-2295-2023, 2023
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This is a critical decade for climate action, but there is no annual tracking of the level of human-induced warming. We build on the Intergovernmental Panel on Climate Change assessment reports that are authoritative but published infrequently to create a set of key global climate indicators that can be tracked through time. Our hope is that this becomes an important annual publication that policymakers, media, scientists and the public can refer to.
Sara Arioli, Ghislain Picard, Laurent Arnaud, and Vincent Favier
The Cryosphere, 17, 2323–2342, https://doi.org/10.5194/tc-17-2323-2023, https://doi.org/10.5194/tc-17-2323-2023, 2023
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To assess the drivers of the snow grain size evolution during snow drift, we exploit a 5-year time series of the snow grain size retrieved from spectral-albedo observations made with a new, autonomous, multi-band radiometer and compare it to observations of snow drift, snowfall and snowmelt at a windy location of coastal Antarctica. Our results highlight the complexity of the grain size evolution in the presence of snow drift and show an overall tendency of snow drift to limit its variations.
Simone Ventisette, Samuele Baldini, Claudio Artoni, Silvia Becagli, Laura Caiazzo, Barbara Delmonte, Massimo Frezzotti, Raffaello Nardin, Joel Savarino, Mirko Severi, Andrea Spolaor, Barbara Stenni, and Rita Traversi
EGUsphere, https://doi.org/10.5194/egusphere-2023-393, https://doi.org/10.5194/egusphere-2023-393, 2023
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The paper reports the spatial variability of concentration and fluxes of chemical impurities in superficial snow over unexplored area of the East Antarctic ice sheet. Pinatubo and Puyehue-Cordón Caulle volcanic eruptions in non-sea salt sulfate and dust snow pits record were used to achieve the accumulation rates. Deposition (wet, dry and uptake from snow surface) and post deposition processes are constrained. These knowledges are fundamental in Antarctic ice cores stratigraphies interpretation.
Romilly Harris Stuart, Anne-Katrine Faber, Sonja Wahl, Maria Hörhold, Sepp Kipfstuhl, Kristian Vasskog, Melanie Behrens, Alexandra M. Zuhr, and Hans Christian Steen-Larsen
The Cryosphere, 17, 1185–1204, https://doi.org/10.5194/tc-17-1185-2023, https://doi.org/10.5194/tc-17-1185-2023, 2023
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This empirical study uses continuous daily measurements from the Greenland Ice Sheet to document changes in surface snow properties. Consistent changes in snow isotopic composition are observed in the absence of deposition due to surface processes, indicating the isotopic signal of deposited precipitation is not always preserved. Our observations have potential implications for the interpretation of water isotopes in ice cores – historically assumed to reflect isotopic composition at deposition.
Niccolò Maffezzoli, Eliza Cook, Willem G. M. van der Bilt, Eivind N. Støren, Daniela Festi, Florian Muthreich, Alistair W. R. Seddon, François Burgay, Giovanni Baccolo, Amalie R. F. Mygind, Troels Petersen, Andrea Spolaor, Sebastiano Vascon, Marcello Pelillo, Patrizia Ferretti, Rafael S. dos Reis, Jefferson C. Simões, Yuval Ronen, Barbara Delmonte, Marco Viccaro, Jørgen Peder Steffensen, Dorthe Dahl-Jensen, Kerim H. Nisancioglu, and Carlo Barbante
The Cryosphere, 17, 539–565, https://doi.org/10.5194/tc-17-539-2023, https://doi.org/10.5194/tc-17-539-2023, 2023
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Multiple lines of research in ice core science are limited by manually intensive and time-consuming optical microscopy investigations for the detection of insoluble particles, from pollen grains to volcanic shards. To help overcome these limitations and support researchers, we present a novel methodology for the identification and autonomous classification of ice core insoluble particles based on flow image microscopy and neural networks.
François Burgay, Rafael Pedro Fernández, Delia Segato, Clara Turetta, Christopher S. Blaszczak-Boxe, Rachael H. Rhodes, Claudio Scarchilli, Virginia Ciardini, Carlo Barbante, Alfonso Saiz-Lopez, and Andrea Spolaor
The Cryosphere, 17, 391–405, https://doi.org/10.5194/tc-17-391-2023, https://doi.org/10.5194/tc-17-391-2023, 2023
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The paper presents the first ice-core record of bromine (Br) in the Antarctic plateau. By the observation of the ice core and the application of atmospheric chemical models, we investigate the behaviour of bromine after its deposition into the snowpack, with interest in the effect of UV radiation change connected to the formation of the ozone hole, the role of volcanic deposition, and the possible use of Br to reconstruct past sea ice changes from ice core collect in the inner Antarctic plateau.
Wiebke Scholz, Jiali Shen, Diego Aliaga, Cheng Wu, Samara Carbone, Isabel Moreno, Qiaozhi Zha, Wei Huang, Liine Heikkinen, Jean Luc Jaffrezo, Gaelle Uzu, Eva Partoll, Markus Leiminger, Fernando Velarde, Paolo Laj, Patrick Ginot, Paolo Artaxo, Alfred Wiedensohler, Markku Kulmala, Claudia Mohr, Marcos Andrade, Victoria Sinclair, Federico Bianchi, and Armin Hansel
Atmos. Chem. Phys., 23, 895–920, https://doi.org/10.5194/acp-23-895-2023, https://doi.org/10.5194/acp-23-895-2023, 2023
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Dimethyl sulfide (DMS), emitted from the ocean, is the most abundant biogenic sulfur emission into the atmosphere. OH radicals, among others, can oxidize DMS to sulfuric and methanesulfonic acid, which are relevant for aerosol formation. We quantified DMS and nearly all DMS oxidation products with novel mass spectrometric instruments for gas and particle phase at the high mountain station Chacaltaya (5240 m a.s.l.) in the Bolivian Andes in free tropospheric air after long-range transport.
Xavier Giraud, Mélanie Baroni, and Rita Traversi
EGUsphere, https://doi.org/10.5194/egusphere-2022-1455, https://doi.org/10.5194/egusphere-2022-1455, 2023
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The snowpack in High Antarctic Plateau is an interface medium between the atmosphere and the firn, where past climate conditions are recorded. Originating mainly from oceanic sources, chlorine is deposited along with snow. We propose a mechanism implying the diffusion of HCl at the scale of snow grains, longing a few decades for its release to the Antarctic atmosphere. Based on this scenario, the fate of the anthropogenic 36Cl originating from the nuclear tests can be forcasted.
Ghislain Picard, Marion Leduc-Leballeur, Alison F. Banwell, Ludovic Brucker, and Giovanni Macelloni
The Cryosphere, 16, 5061–5083, https://doi.org/10.5194/tc-16-5061-2022, https://doi.org/10.5194/tc-16-5061-2022, 2022
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Using a snowpack radiative transfer model, we investigate in which conditions meltwater can be detected from passive microwave satellite observations from 1.4 to 37 GHz. In particular, we determine the minimum detectable liquid water content, the maximum depth of detection of a buried wet snow layer and the risk of false alarm due to supraglacial lakes. These results provide information for the developers of new, more advanced satellite melt products and for the users of the existing products.
Pete D. Akers, Joël Savarino, Nicolas Caillon, Olivier Magand, and Emmanuel Le Meur
Atmos. Chem. Phys., 22, 15637–15657, https://doi.org/10.5194/acp-22-15637-2022, https://doi.org/10.5194/acp-22-15637-2022, 2022
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Nitrate isotopes in Antarctic ice do not preserve the seasonal isotopic cycles of the atmosphere, which limits their use to study the past. We studied nitrate along an 850 km Antarctic transect to learn how these cycles are changed by sunlight-driven chemistry in the snow. Our findings suggest that the snow accumulation rate and other environmental signals can be extracted from nitrate with the right sampling and analytical approaches.
Dominic Saunderson, Andrew Mackintosh, Felicity McCormack, Richard Selwyn Jones, and Ghislain Picard
The Cryosphere, 16, 4553–4569, https://doi.org/10.5194/tc-16-4553-2022, https://doi.org/10.5194/tc-16-4553-2022, 2022
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We investigate the variability in surface melt on the Shackleton Ice Shelf in East Antarctica over the last 2 decades (2003–2021). Using daily satellite observations and the machine learning approach of a self-organising map, we identify nine distinct spatial patterns of melt. These patterns allow comparisons of melt within and across melt seasons and highlight the importance of both air temperatures and local controls such as topography, katabatic winds, and albedo in driving surface melt.
Yanzhi Cao, Zhuang Jiang, Becky Alexander, Jihong Cole-Dai, Joel Savarino, Joseph Erbland, and Lei Geng
Atmos. Chem. Phys., 22, 13407–13422, https://doi.org/10.5194/acp-22-13407-2022, https://doi.org/10.5194/acp-22-13407-2022, 2022
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We investigate the potential of ice-core preserved nitrate isotopes as proxies of stratospheric ozone variability by measuring nitrate isotopes in a shallow ice core from the South Pole. The large variability in the snow accumulation rate and its slight increase after the 1970s masked any signals caused by the ozone hole. Moreover, the nitrate oxygen isotope decrease may reflect changes in the atmospheric oxidation environment in the Southern Ocean.
Antoine Grisart, Mathieu Casado, Vasileios Gkinis, Bo Vinther, Philippe Naveau, Mathieu Vrac, Thomas Laepple, Bénédicte Minster, Frederic Prié, Barbara Stenni, Elise Fourré, Hans Christian Steen-Larsen, Jean Jouzel, Martin Werner, Katy Pol, Valérie Masson-Delmotte, Maria Hoerhold, Trevor Popp, and Amaelle Landais
Clim. Past, 18, 2289–2301, https://doi.org/10.5194/cp-18-2289-2022, https://doi.org/10.5194/cp-18-2289-2022, 2022
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This paper presents a compilation of high-resolution (11 cm) water isotopic records, including published and new measurements, for the last 800 000 years from the EPICA Dome C ice core, Antarctica. Using this new combined water isotopes (δ18O and δD) dataset, we study the variability and possible influence of diffusion at the multi-decadal to multi-centennial scale. We observe a stronger variability at the onset of the interglacial interval corresponding to a warm period.
Ghislain Picard, Henning Löwe, and Christian Mätzler
The Cryosphere, 16, 3861–3866, https://doi.org/10.5194/tc-16-3861-2022, https://doi.org/10.5194/tc-16-3861-2022, 2022
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Microwave satellite observations used to monitor the cryosphere require radiative transfer models for their interpretation. These models represent how microwaves are scattered by snow and ice. However no existing theory is suitable for all types of snow and ice found on Earth. We adapted a recently published generic scattering theory to snow and show how it may improve the representation of snows with intermediate densities (~500 kg/m3) and/or with coarse grains at high microwave frequencies.
Albane Barbero, Roberto Grilli, Markus M. Frey, Camille Blouzon, Detlev Helmig, Nicolas Caillon, and Joël Savarino
Atmos. Chem. Phys., 22, 12025–12054, https://doi.org/10.5194/acp-22-12025-2022, https://doi.org/10.5194/acp-22-12025-2022, 2022
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The high reactivity of the summer Antarctic boundary layer results in part from the emissions of nitrogen oxides produced during photo-denitrification of the snowpack, but its underlying mechanisms are not yet fully understood. The results of this study suggest that more NO2 is produced from the snowpack early in the photolytic season, possibly due to stronger UV irradiance caused by a smaller solar zenith angle near the solstice.
Gauthier Vérin, Florent Domine, Marcel Babin, Ghislain Picard, and Laurent Arnaud
The Cryosphere, 16, 3431–3449, https://doi.org/10.5194/tc-16-3431-2022, https://doi.org/10.5194/tc-16-3431-2022, 2022
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Snow physical properties on Arctic sea ice are monitored during the melt season. As snow grains grow, and the snowpack thickness is reduced, the surface albedo decreases. The extra absorbed energy accelerates melting. Radiative transfer modeling shows that more radiation is then transmitted to the snow–sea-ice interface. A sharp increase in transmitted radiation takes place when the snowpack thins significantly, and this coincides with the initiation of the phytoplankton bloom in the seawater.
Carlton Xavier, Metin Baykara, Robin Wollesen de Jonge, Barbara Altstädter, Petri Clusius, Ville Vakkari, Roseline Thakur, Lisa Beck, Silvia Becagli, Mirko Severi, Rita Traversi, Radovan Krejci, Peter Tunved, Mauro Mazzola, Birgit Wehner, Mikko Sipilä, Markku Kulmala, Michael Boy, and Pontus Roldin
Atmos. Chem. Phys., 22, 10023–10043, https://doi.org/10.5194/acp-22-10023-2022, https://doi.org/10.5194/acp-22-10023-2022, 2022
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The focus of this work is to study and improve our understanding of processes involved in the formation and growth of new particles in a remote Arctic marine environment. We run the 1D model ADCHEM along air mass trajectories arriving at Ny-Ålesund in May 2018. The model finds that ion-mediated H2SO4–NH3 nucleation can explain the observed new particle formation at Ny-Ålesund. The growth of particles is driven via H2SO4 condensation and formation of methane sulfonic acid in the aqueous phase.
Fabio Giardi, Silvia Nava, Giulia Calzolai, Giulia Pazzi, Massimo Chiari, Andrea Faggi, Bianca Patrizia Andreini, Chiara Collaveri, Elena Franchi, Guido Nincheri, Alessandra Amore, Silvia Becagli, Mirko Severi, Rita Traversi, and Franco Lucarelli
Atmos. Chem. Phys., 22, 9987–10005, https://doi.org/10.5194/acp-22-9987-2022, https://doi.org/10.5194/acp-22-9987-2022, 2022
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The restriction measures adopted to contain the COVID-19 virus offered a unique opportunity to study urban particulate emissions in the near absence of traffic, which is one of the main emission sources in the urban environment. However, the drastic decrease in this source of particulate matter during the months of national lockdown did not lead to an equal decrease in the total particulate load. This is due to the inverse behavior shown by different sources, especially secondary sources.
Silvia Becagli, Elena Barbaro, Simone Bonamano, Laura Caiazzo, Alcide di Sarra, Matteo Feltracco, Paolo Grigioni, Jost Heintzenberg, Luigi Lazzara, Michel Legrand, Alice Madonia, Marco Marcelli, Chiara Melillo, Daniela Meloni, Caterina Nuccio, Giandomenico Pace, Ki-Tae Park, Suzanne Preunkert, Mirko Severi, Marco Vecchiato, Roberta Zangrando, and Rita Traversi
Atmos. Chem. Phys., 22, 9245–9263, https://doi.org/10.5194/acp-22-9245-2022, https://doi.org/10.5194/acp-22-9245-2022, 2022
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Measurements of phytoplanktonic dimethylsulfide and its oxidation products in the Antarctic atmosphere allow us to understand the role of the oceanic (sea ice melting, Chl α and dimethylsulfoniopropionate) and atmospheric (wind direction and speed, humidity, solar radiation and transport processes) factors in the biogenic aerosol formation, concentration and characteristic ratio between components in an Antarctic coastal site facing the polynya of the Ross Sea.
Zhuang Jiang, Joel Savarino, Becky Alexander, Joseph Erbland, Jean-Luc Jaffrezo, and Lei Geng
The Cryosphere, 16, 2709–2724, https://doi.org/10.5194/tc-16-2709-2022, https://doi.org/10.5194/tc-16-2709-2022, 2022
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A record of year-round atmospheric nitrate isotopic composition along with snow nitrate isotopic data from Summit, Greenland, revealed apparent enrichments in nitrogen isotopes in snow nitrate compared to atmospheric nitrate, in addition to a relatively smaller degree of changes in oxygen isotopes. The results suggest that at this site post-depositional processing takes effect, which should be taken into account when interpreting ice-core nitrate isotope records.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Saehee Lim, Meehye Lee, Joel Savarino, and Paolo Laj
Atmos. Chem. Phys., 22, 5099–5115, https://doi.org/10.5194/acp-22-5099-2022, https://doi.org/10.5194/acp-22-5099-2022, 2022
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We determined δ15N(NO3−) and Δ17O(NO3−) of PM2.5 in Seoul during 2018–2019 and estimated quantitatively the contribution of oxidation pathways to NO3− formation and NOx emission sources. The nighttime pathway played a significant role in NO3− formation during the winter, and its contribution further increased up to 70 % on haze days when PM2.5 was greater than 75 µg m−3. Vehicle emissions were confirmed as a main NO3− source with an increasing contribution from coal combustion in winter.
Aki Virkkula, Henrik Grythe, John Backman, Tuukka Petäjä, Maurizio Busetto, Christian Lanconelli, Angelo Lupi, Silvia Becagli, Rita Traversi, Mirko Severi, Vito Vitale, Patrick Sheridan, and Elisabeth Andrews
Atmos. Chem. Phys., 22, 5033–5069, https://doi.org/10.5194/acp-22-5033-2022, https://doi.org/10.5194/acp-22-5033-2022, 2022
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Optical properties of surface aerosols at Dome C, Antarctica, in 2007–2013 and their potential source areas are presented. The equivalent black carbon (eBC) mass concentrations were compared with eBC measured at three other Antarctic sites: the South Pole (SPO) and two coastal sites, Neumayer and Syowa. Transport analysis suggests that South American BC emissions are the largest contributor to eBC at Dome C.
Tobias Erhardt, Matthias Bigler, Urs Federer, Gideon Gfeller, Daiana Leuenberger, Olivia Stowasser, Regine Röthlisberger, Simon Schüpbach, Urs Ruth, Birthe Twarloh, Anna Wegner, Kumiko Goto-Azuma, Takayuki Kuramoto, Helle A. Kjær, Paul T. Vallelonga, Marie-Louise Siggaard-Andersen, Margareta E. Hansson, Ailsa K. Benton, Louise G. Fleet, Rob Mulvaney, Elizabeth R. Thomas, Nerilie Abram, Thomas F. Stocker, and Hubertus Fischer
Earth Syst. Sci. Data, 14, 1215–1231, https://doi.org/10.5194/essd-14-1215-2022, https://doi.org/10.5194/essd-14-1215-2022, 2022
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The datasets presented alongside this manuscript contain high-resolution concentration measurements of chemical impurities in deep ice cores, NGRIP and NEEM, from the Greenland ice sheet. The impurities originate from the deposition of aerosols to the surface of the ice sheet and are influenced by source, transport and deposition processes. Together, these records contain detailed, multi-parameter records of past climate variability over the last glacial period.
Jiamei Lin, Anders Svensson, Christine S. Hvidberg, Johannes Lohmann, Steffen Kristiansen, Dorthe Dahl-Jensen, Jørgen Peder Steffensen, Sune Olander Rasmussen, Eliza Cook, Helle Astrid Kjær, Bo M. Vinther, Hubertus Fischer, Thomas Stocker, Michael Sigl, Matthias Bigler, Mirko Severi, Rita Traversi, and Robert Mulvaney
Clim. Past, 18, 485–506, https://doi.org/10.5194/cp-18-485-2022, https://doi.org/10.5194/cp-18-485-2022, 2022
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We employ acidity records from Greenland and Antarctic ice cores to estimate the emission strength, frequency and climatic forcing for large volcanic eruptions from the last half of the last glacial period. A total of 25 volcanic eruptions are found to be larger than any eruption in the last 2500 years, and we identify more eruptions than obtained from geological evidence. Towards the end of the glacial period, there is a notable increase in volcanic activity observed for Greenland.
Marjan Marbouti, Sehyun Jang, Silvia Becagli, Gabriel Navarro, Rita Traversi, Kitack Lee, Tuomo Nieminen, Lisa J. Beck, Markku Kulmala, Veli-Matti Kerminen, and Mikko Sipilä
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-52, https://doi.org/10.5194/acp-2022-52, 2022
Publication in ACP not foreseen
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This research was done to understand and investigate the roles of Chl-a, PP and sea ice extent in controlling and producing the in-situ measured MSA, SA, HIO3, HOM and aerosol concentrations over the Greenland and Barents Seas. Our results provide strong support to the hypothesis that MSA, SA and small-particle concentrations in the Svalbard area are directly linked to ocean biological activity and sea ice melting during springtime.
Julia Schmale, Sangeeta Sharma, Stefano Decesari, Jakob Pernov, Andreas Massling, Hans-Christen Hansson, Knut von Salzen, Henrik Skov, Elisabeth Andrews, Patricia K. Quinn, Lucia M. Upchurch, Konstantinos Eleftheriadis, Rita Traversi, Stefania Gilardoni, Mauro Mazzola, James Laing, and Philip Hopke
Atmos. Chem. Phys., 22, 3067–3096, https://doi.org/10.5194/acp-22-3067-2022, https://doi.org/10.5194/acp-22-3067-2022, 2022
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Long-term data sets of Arctic aerosol properties from 10 stations across the Arctic provide evidence that anthropogenic influence on the Arctic atmospheric chemical composition has declined in winter, a season which is typically dominated by mid-latitude emissions. The number of significant trends in summer is smaller than in winter, and overall the pattern is ambiguous with some significant positive and negative trends. This reflects the mixed influence of natural and anthropogenic emissions.
Nicolas Stoll, Maria Hörhold, Tobias Erhardt, Jan Eichler, Camilla Jensen, and Ilka Weikusat
The Cryosphere, 16, 667–688, https://doi.org/10.5194/tc-16-667-2022, https://doi.org/10.5194/tc-16-667-2022, 2022
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We mapped and analysed solid inclusion in the upper 1340 m of the EGRIP ice core with Raman spectroscopy and microstructure mapping, based on bulk dust content derived via continuous flow analysis. We observe a large variety in mineralogy throughout the core and samples. The main minerals are sulfates, especially gypsum, and terrestrial dust minerals, such as quartz, mica, and feldspar. A change in mineralogy occurs around 900 m depth indicating a climate-related imprint.
Alvaro Robledano, Ghislain Picard, Laurent Arnaud, Fanny Larue, and Inès Ollivier
The Cryosphere, 16, 559–579, https://doi.org/10.5194/tc-16-559-2022, https://doi.org/10.5194/tc-16-559-2022, 2022
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Topography controls the surface temperature of snow-covered, mountainous areas. We developed a modelling chain that uses ray-tracing methods to quantify the impact of a few topographic effects on snow surface temperature at high spatial resolution. Its large spatial and temporal variations are correctly simulated over a 50 km2 area in the French Alps, and our results show that excluding a single topographic effect results in cooling (or warming) effects on the order of 1 °C.
Nicolas Stoll, Jan Eichler, Maria Hörhold, Tobias Erhardt, Camilla Jensen, and Ilka Weikusat
The Cryosphere, 15, 5717–5737, https://doi.org/10.5194/tc-15-5717-2021, https://doi.org/10.5194/tc-15-5717-2021, 2021
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We did a systematic analysis of the location of inclusions in the EGRIP ice core, the first ice core from an ice stream. We combine this with crystal orientation and grain size data, enabling the first overview about the microstructure of this unique ice core. Micro-inclusions show a strong spatial variability and patterns (clusters or horizontal layers); roughly one-third is located at grain boundaries. More holistic approaches are needed to understand deformation processes in the ice better.
Maria Belke-Brea, Florent Domine, Ghislain Picard, Mathieu Barrere, and Laurent Arnaud
Biogeosciences, 18, 5851–5869, https://doi.org/10.5194/bg-18-5851-2021, https://doi.org/10.5194/bg-18-5851-2021, 2021
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Expanding shrubs in the Arctic change snowpacks into a mix of snow, impurities and buried branches. Snow is a translucent medium into which light penetrates and gets partly absorbed by branches or impurities. Measurements of light attenuation in snow in Northern Quebec, Canada, showed (1) black-carbon-dominated light attenuation in snowpacks without shrubs and (2) buried branches influence radiation attenuation in snow locally, leading to melting and pockets of large crystals close to branches.
Abigail G. Hughes, Sonja Wahl, Tyler R. Jones, Alexandra Zuhr, Maria Hörhold, James W. C. White, and Hans Christian Steen-Larsen
The Cryosphere, 15, 4949–4974, https://doi.org/10.5194/tc-15-4949-2021, https://doi.org/10.5194/tc-15-4949-2021, 2021
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Water isotope records in Greenland and Antarctic ice cores are a valuable proxy for paleoclimate reconstruction and are traditionally thought to primarily reflect precipitation input. However,
post-depositional processes are hypothesized to contribute to the isotope climate signal. In this study we use laboratory experiments, field experiments, and modeling to show that sublimation and vapor–snow isotope exchange can rapidly influence the isotopic composition of the snowpack.
Alexandra M. Zuhr, Thomas Münch, Hans Christian Steen-Larsen, Maria Hörhold, and Thomas Laepple
The Cryosphere, 15, 4873–4900, https://doi.org/10.5194/tc-15-4873-2021, https://doi.org/10.5194/tc-15-4873-2021, 2021
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Firn and ice cores are used to infer past temperatures. However, the imprint of the climatic signal in stable water isotopes is influenced by depositional modifications. We present and use a photogrammetry structure-from-motion approach and find variability in the amount, the timing, and the location of snowfall. Depositional modifications of the surface are observed, leading to mixing of snow from different snowfall events and spatial locations and thus creating noise in the proxy record.
Laura Crick, Andrea Burke, William Hutchison, Mika Kohno, Kathryn A. Moore, Joel Savarino, Emily A. Doyle, Sue Mahony, Sepp Kipfstuhl, James W. B. Rae, Robert C. J. Steele, R. Stephen J. Sparks, and Eric W. Wolff
Clim. Past, 17, 2119–2137, https://doi.org/10.5194/cp-17-2119-2021, https://doi.org/10.5194/cp-17-2119-2021, 2021
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The ~ 74 ka eruption of Toba was one of the largest eruptions of the last 100 ka. We have measured the sulfur isotopic composition for 11 Toba eruption candidates in two Antarctic ice cores. Sulfur isotopes allow us to distinguish between large eruptions that have erupted material into the stratosphere and smaller ones that reach lower altitudes. Using this we have identified the events most likely to be Toba and place the eruption on the transition into a cold period in the Northern Hemisphere.
Raffaello Nardin, Mirko Severi, Alessandra Amore, Silvia Becagli, Francois Burgay, Laura Caiazzo, Virginia Ciardini, Giuliano Dreossi, Massimo Frezzotti, Sang-Bum Hong, Ishaq Khan, Bianca Maria Narcisi, Marco Proposito, Claudio Scarchilli, Enricomaria Selmo, Andrea Spolaor, Barbara Stenni, and Rita Traversi
Clim. Past, 17, 2073–2089, https://doi.org/10.5194/cp-17-2073-2021, https://doi.org/10.5194/cp-17-2073-2021, 2021
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The first step to exploit all the potential information buried in ice cores is to produce a reliable age scale. Based on chemical and isotopic records from the 197 m Antarctic GV7(B) ice core, accurate dating was achieved and showed that the archive spans roughly the last 830 years. The relatively high accumulation rate allowed us to use the non-sea-salt sulfate seasonal pattern to count annual layers. The accumulation rate reconstruction exhibited a slight increase since the 18th century.
Saeid Bagheri Dastgerdi, Melanie Behrens, Jean-Louis Bonne, Maria Hörhold, Gerrit Lohmann, Elisabeth Schlosser, and Martin Werner
The Cryosphere, 15, 4745–4767, https://doi.org/10.5194/tc-15-4745-2021, https://doi.org/10.5194/tc-15-4745-2021, 2021
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In this study, for the first time, water vapour isotope measurements in Antarctica for all seasons of a year are performed. Local temperature is identified as the main driver of δ18O and δD variability. A similar slope of the temperature–δ18O relationship in vapour and surface snow points to the water vapour isotope content as a potential key driver. This dataset can be used as a new dataset to evaluate the capability of isotope-enhanced climate models.
Matteo Rinaldi, Naruki Hiranuma, Gianni Santachiara, Mauro Mazzola, Karam Mansour, Marco Paglione, Cheyanne A. Rodriguez, Rita Traversi, Silvia Becagli, David Cappelletti, and Franco Belosi
Atmos. Chem. Phys., 21, 14725–14748, https://doi.org/10.5194/acp-21-14725-2021, https://doi.org/10.5194/acp-21-14725-2021, 2021
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This study aims to add to the still scant ice-nucleating particle (INP) observations in the Arctic environment, investigating INP concentrations and potential sources, during spring and summertime, at the ground-level site of GVB. The lack of a clear concentration seasonal trend, in contrast with previous works, shows an important interannual variability of Arctic INP sources, which may be both terrestrial and marine, outside the Arctic haze period.
Federico Dallo, Daniele Zannoni, Jacopo Gabrieli, Paolo Cristofanelli, Francescopiero Calzolari, Fabrizio de Blasi, Andrea Spolaor, Dario Battistel, Rachele Lodi, Warren Raymond Lee Cairns, Ann Mari Fjæraa, Paolo Bonasoni, and Carlo Barbante
Atmos. Meas. Tech., 14, 6005–6021, https://doi.org/10.5194/amt-14-6005-2021, https://doi.org/10.5194/amt-14-6005-2021, 2021
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Our work showed how the adoption of low-cost technology could be useful in environmental research and monitoring. We focused our work on tropospheric ozone, but we also showed how to make a general purpose low-cost sensing system which may be adapted and optimised to be used in many other case studies. Given the importance of providing quality data, we put a lot of effort in the sensor's calibration, and we believe that our results show how to exploit the potential of the low-cost technology.
Zhuang Jiang, Becky Alexander, Joel Savarino, Joseph Erbland, and Lei Geng
The Cryosphere, 15, 4207–4220, https://doi.org/10.5194/tc-15-4207-2021, https://doi.org/10.5194/tc-15-4207-2021, 2021
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We used a snow photochemistry model (TRANSITS) to simulate the seasonal nitrate snow profile at Summit, Greenland. Comparisons between model outputs and observations suggest that at Summit post-depositional processing is active and probably dominates the snowpack δ15N seasonality. We also used the model to assess the degree of snow nitrate loss and the consequences in its isotopes at present and in the past, which helps for quantitative interpretations of ice-core nitrate records.
Michele Bertò, David Cappelletti, Elena Barbaro, Cristiano Varin, Jean-Charles Gallet, Krzysztof Markowicz, Anna Rozwadowska, Mauro Mazzola, Stefano Crocchianti, Luisa Poto, Paolo Laj, Carlo Barbante, and Andrea Spolaor
Atmos. Chem. Phys., 21, 12479–12493, https://doi.org/10.5194/acp-21-12479-2021, https://doi.org/10.5194/acp-21-12479-2021, 2021
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We present the daily and seasonal variability in black carbon (BC) in surface snow inferred from two specific experiments based on the hourly and daily time resolution sampling during the Arctic spring in Svalbard. These unique data sets give us, for the first time, the opportunity to evaluate the associations between the observed surface snow BC mass concentration and a set of predictors corresponding to the considered meteorological and snow physico-chemical parameters.
Helle Astrid Kjær, Lisa Lolk Hauge, Marius Simonsen, Zurine Yoldi, Iben Koldtoft, Maria Hörhold, Johannes Freitag, Sepp Kipfstuhl, Anders Svensson, and Paul Vallelonga
The Cryosphere, 15, 3719–3730, https://doi.org/10.5194/tc-15-3719-2021, https://doi.org/10.5194/tc-15-3719-2021, 2021
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Ice core analyses are often done in home laboratories after costly transport of samples from the field. This limits the amount of sample that can be analysed.
Here, we present the first truly field-portable continuous flow analysis (CFA) system for the analysis of impurities in snow, firn and ice cores while still in the field: the lightweight in situ analysis (LISA) box.
LISA is demonstrated in Greenland to reconstruct accumulation, conductivity and peroxide in snow cores.
Congbo Song, Manuel Dall'Osto, Angelo Lupi, Mauro Mazzola, Rita Traversi, Silvia Becagli, Stefania Gilardoni, Stergios Vratolis, Karl Espen Yttri, David C. S. Beddows, Julia Schmale, James Brean, Agung Ghani Kramawijaya, Roy M. Harrison, and Zongbo Shi
Atmos. Chem. Phys., 21, 11317–11335, https://doi.org/10.5194/acp-21-11317-2021, https://doi.org/10.5194/acp-21-11317-2021, 2021
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We present a cluster analysis of relatively long-term (2015–2019) aerosol aerodynamic volume size distributions up to 20 μm in the Arctic for the first time. The study found that anthropogenic and natural aerosols comprised 27 % and 73 % of the occurrence of the coarse-mode aerosols, respectively. Our study shows that about two-thirds of the coarse-mode aerosols are related to two sea-spray-related aerosol clusters, indicating that sea spray aerosol may more complex in the Arctic environment.
Delia Segato, Maria Del Carmen Villoslada Hidalgo, Ross Edwards, Elena Barbaro, Paul Vallelonga, Helle Astrid Kjær, Marius Simonsen, Bo Vinther, Niccolò Maffezzoli, Roberta Zangrando, Clara Turetta, Dario Battistel, Orri Vésteinsson, Carlo Barbante, and Andrea Spolaor
Clim. Past, 17, 1533–1545, https://doi.org/10.5194/cp-17-1533-2021, https://doi.org/10.5194/cp-17-1533-2021, 2021
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Human influence on fire regimes in the past is poorly understood, especially at high latitudes. We present 5 kyr of fire proxies levoglucosan, black carbon, and ammonium in the RECAP ice core in Greenland and reconstruct for the first time the fire regime in the high North Atlantic region, comprising coastal east Greenland and Iceland. Climate is the main driver of the fire regime, but at 1.1 kyr BP a contribution may be made by the deforestation resulting from Viking colonization of Iceland.
Sarah Albertin, Joël Savarino, Slimane Bekki, Albane Barbero, and Nicolas Caillon
Atmos. Chem. Phys., 21, 10477–10497, https://doi.org/10.5194/acp-21-10477-2021, https://doi.org/10.5194/acp-21-10477-2021, 2021
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We report an efficient method to collect atmospheric NO2 adapted for multi-isotopic analysis and present the first NO2 triple oxygen and double nitrogen isotope measurements. Atmospheric samplings carried out in Grenoble, France, highlight the NO2 isotopic signature sensitivity to the local NOx emissions and chemical regimes. These preliminary results are very promising for using the combination of Δ17O and δ15N of NO2 as a probe of the atmospheric NOx emissions and chemistry.
Sehyun Jang, Ki-Tae Park, Kitack Lee, Young Jun Yoon, Kitae Kim, Hyun Young Chung, Eunho Jang, Silvia Becagli, Bang Yong Lee, Rita Traversi, Konstantinos Eleftheriadis, Radovan Krejci, and Ove Hermansen
Atmos. Chem. Phys., 21, 9761–9777, https://doi.org/10.5194/acp-21-9761-2021, https://doi.org/10.5194/acp-21-9761-2021, 2021
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This study provides comprehensive datasets encompassing seasonal and interannual variations in sulfate and MSA concentration in aerosol particles in the Arctic atmosphere. As oxidation products of DMS have important roles in new particle formation and growth, we focused on factors affecting their variability and the branching ratio of DMS oxidation. We found a strong correlation between the ratio and the light condition, chemical properties of particles, and biological activities near Svalbard.
Cited articles
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Short summary
This work presents a new approach to the estimation of accumulation rates at Concordia Station, East-Antarctica, for the last 20 years, from a new data set of chemical tracers and snow micro-scale properties measured in a snow trench. Multi-annual and meter to decameter scale variability of accumulation rates are compared again in-situ measurements of surface laser scanner and stake farm, with very good agreement. This further constrains SMB estimation for Antarctica at high temporal resolution.
This work presents a new approach to the estimation of accumulation rates at Concordia Station,...