Articles | Volume 15, issue 4
https://doi.org/10.5194/tc-15-2001-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/tc-15-2001-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Apr 2021
Research article |
| 23 Apr 2021
| 23 Apr 2021
Interfacial supercooling and the precipitation of hydrohalite in frozen NaCl solutions as seen by X-ray absorption spectroscopy
Thorsten Bartels-Rausch
CORRESPONDING AUTHOR
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
Xiangrui Kong
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
now at: Department of Chemistry and Molecular Biology, Atmospheric
Science, University of Gothenburg, Gothenburg, Sweden
Fabrizio Orlando
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
now at: Omya International AG, Oftringen, Switzerland
Luca Artiglia
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
Astrid Waldner
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
Thomas Huthwelker
Swiss Light Source (SLS), Paul Scherrer Institut, Villigen PSI,
Switzerland
Markus Ammann
Laboratory of Environmental Chemistry, Paul Scherrer Institut,
Villigen PSI, Switzerland
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Hannah Meusel, Yasin Elshorbany, Uwe Kuhn, Thorsten Bartels-Rausch, Kathrin Reinmuth-Selzle, Christopher J. Kampf, Guo Li, Xiaoxiang Wang, Jos Lelieveld, Ulrich Pöschl, Thorsten Hoffmann, Hang Su, Markus Ammann, and Yafang Cheng
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Thomas Berkemeier, Markus Ammann, Ulrich K. Krieger, Thomas Peter, Peter Spichtinger, Ulrich Pöschl, Manabu Shiraiwa, and Andrew J. Huisman
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Goran Gržinić, Thorsten Bartels-Rausch, Andreas Türler, and Markus Ammann
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Pascale S. J. Lakey, Thomas Berkemeier, Manuel Krapf, Josef Dommen, Sarah S. Steimer, Lisa K. Whalley, Trevor Ingham, Maria T. Baeza-Romero, Ulrich Pöschl, Manabu Shiraiwa, Markus Ammann, and Dwayne E. Heard
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Laura González Palacios, Pablo Corral Arroyo, Kifle Z. Aregahegn, Sarah S. Steimer, Thorsten Bartels-Rausch, Barbara Nozière, Christian George, Markus Ammann, and Rainer Volkamer
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Guo Li, Hang Su, Xin Li, Uwe Kuhn, Hannah Meusel, Thorsten Hoffmann, Markus Ammann, Ulrich Pöschl, Min Shao, and Yafang Cheng
Atmos. Chem. Phys., 16, 10299–10311, https://doi.org/10.5194/acp-16-10299-2016, https://doi.org/10.5194/acp-16-10299-2016, 2016
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Indoor and outdoor formaldehyde (HCHO) are both of considerable concern because of its health effects and its role in atmospheric chemistry. The heterogeneous reactions between gaseous HCHO with soils can pose important impact on both HCHO budget and soil ecosystem. Our results confirms that HCHO uptake by soil is a complex process involving both adsorption/desorption and chemical reactions. Soil and soil-derived airborne particles can either act as a source or a sink for HCHO.
G. Gržinić, T. Bartels-Rausch, T. Berkemeier, A. Türler, and M. Ammann
Atmos. Chem. Phys., 15, 13615–13625, https://doi.org/10.5194/acp-15-13615-2015, https://doi.org/10.5194/acp-15-13615-2015, 2015
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S. S. Steimer, U. K. Krieger, Y.-F. Te, D. M. Lienhard, A. J. Huisman, B. P. Luo, M. Ammann, and T. Peter
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E. S. Thomson, X. Kong, P. Papagiannakopoulos, and J. B. C. Pettersson
Atmos. Chem. Phys., 15, 1621–1632, https://doi.org/10.5194/acp-15-1621-2015, https://doi.org/10.5194/acp-15-1621-2015, 2015
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S. S. Steimer, M. Lampimäki, E. Coz, G. Grzinic, and M. Ammann
Atmos. Chem. Phys., 14, 10761–10772, https://doi.org/10.5194/acp-14-10761-2014, https://doi.org/10.5194/acp-14-10761-2014, 2014
M. Legrand, S. Preunkert, M. Frey, Th. Bartels-Rausch, A. Kukui, M. D. King, J. Savarino, M. Kerbrat, and B. Jourdain
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T. Bartels-Rausch, H.-W. Jacobi, T. F. Kahan, J. L. Thomas, E. S. Thomson, J. P. D. Abbatt, M. Ammann, J. R. Blackford, H. Bluhm, C. Boxe, F. Domine, M. M. Frey, I. Gladich, M. I. Guzmán, D. Heger, Th. Huthwelker, P. Klán, W. F. Kuhs, M. H. Kuo, S. Maus, S. G. Moussa, V. F. McNeill, J. T. Newberg, J. B. C. Pettersson, M. Roeselová, and J. R. Sodeau
Atmos. Chem. Phys., 14, 1587–1633, https://doi.org/10.5194/acp-14-1587-2014, https://doi.org/10.5194/acp-14-1587-2014, 2014
M. Ammann, R. A. Cox, J. N. Crowley, M. E. Jenkin, A. Mellouki, M. J. Rossi, J. Troe, and T. J. Wallington
Atmos. Chem. Phys., 13, 8045–8228, https://doi.org/10.5194/acp-13-8045-2013, https://doi.org/10.5194/acp-13-8045-2013, 2013
T. Bartels-Rausch, S. N. Wren, S. Schreiber, F. Riche, M. Schneebeli, and M. Ammann
Atmos. Chem. Phys., 13, 6727–6739, https://doi.org/10.5194/acp-13-6727-2013, https://doi.org/10.5194/acp-13-6727-2013, 2013
T. Berkemeier, A. J. Huisman, M. Ammann, M. Shiraiwa, T. Koop, and U. Pöschl
Atmos. Chem. Phys., 13, 6663–6686, https://doi.org/10.5194/acp-13-6663-2013, https://doi.org/10.5194/acp-13-6663-2013, 2013
E. S. Thomson, X. Kong, N. Marković, P. Papagiannakopoulos, and J. B. C. Pettersson
Atmos. Chem. Phys., 13, 2223–2233, https://doi.org/10.5194/acp-13-2223-2013, https://doi.org/10.5194/acp-13-2223-2013, 2013
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Wind-driven snow redistribution affects glacier mass balance. A case study of Hintereisferner glacier in Austria used high-resolution observations and simulations to model snow redistribution. Simulations matched observations, showing the potential of the model for studying snow redistribution on other mountain glaciers.
Christophe Leroy-Dos Santos, Elise Fourré, Cécile Agosta, Mathieu Casado, Alexandre Cauquoin, Martin Werner, Benedicte Minster, Frédéric Prié, Olivier Jossoud, Leila Petit, and Amaëlle Landais
The Cryosphere, 17, 5241–5254, https://doi.org/10.5194/tc-17-5241-2023, https://doi.org/10.5194/tc-17-5241-2023, 2023
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In the face of global warming, understanding the changing water cycle and temperatures in polar regions is crucial. These factors directly impact the balance of ice sheets in the Arctic and Antarctic. By studying the composition of water vapor, we gain insights into climate variations. Our 2-year study at Dumont d’Urville station, Adélie Land, offers valuable data to refine models. Additionally, we demonstrate how modeling aids in interpreting signals from ice core samples in the region.
Alia L. Khan, Peng Xian, and Joshua P. Schwarz
The Cryosphere, 17, 2909–2918, https://doi.org/10.5194/tc-17-2909-2023, https://doi.org/10.5194/tc-17-2909-2023, 2023
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Ice–albedo feedbacks in the ablation region of the Greenland Ice Sheet are difficult to constrain and model. Surface samples were collected across the 2014 summer melt season from different ice surface colors. On average, concentrations were higher in patches that were visibly dark, compared to medium patches and light patches, suggesting that black carbon aggregation contributed to snow aging, and vice versa. High concentrations are likely due to smoke transport from high-latitude wildfires.
Sara Arioli, Ghislain Picard, Laurent Arnaud, and Vincent Favier
The Cryosphere, 17, 2323–2342, https://doi.org/10.5194/tc-17-2323-2023, https://doi.org/10.5194/tc-17-2323-2023, 2023
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To assess the drivers of the snow grain size evolution during snow drift, we exploit a 5-year time series of the snow grain size retrieved from spectral-albedo observations made with a new, autonomous, multi-band radiometer and compare it to observations of snow drift, snowfall and snowmelt at a windy location of coastal Antarctica. Our results highlight the complexity of the grain size evolution in the presence of snow drift and show an overall tendency of snow drift to limit its variations.
Guillaume Gastineau, Claude Frankignoul, Yongqi Gao, Yu-Chiao Liang, Young-Oh Kwon, Annalisa Cherchi, Rohit Ghosh, Elisa Manzini, Daniela Matei, Jennifer Mecking, Lingling Suo, Tian Tian, Shuting Yang, and Ying Zhang
The Cryosphere, 17, 2157–2184, https://doi.org/10.5194/tc-17-2157-2023, https://doi.org/10.5194/tc-17-2157-2023, 2023
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Snow cover variability is important for many human activities. This study aims to understand the main drivers of snow cover in observations and models in order to better understand it and guide the improvement of climate models and forecasting systems. Analyses reveal a dominant role for sea surface temperature in the Pacific. Winter snow cover is also found to have important two-way interactions with the troposphere and stratosphere. No robust influence of the sea ice concentration is found.
Daniela Brito Melo, Armin Sigmund, and Michael Lehning
EGUsphere, https://doi.org/10.5194/egusphere-2023-488, https://doi.org/10.5194/egusphere-2023-488, 2023
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Snow saltation – the transport of snow close to the surface – occurs when the wind blows over a snow covered surface with sufficient strength. This phenomenon is represented in several climate models, however, with a limited accuracy. By performing numerical simulations and a detailed analysis of previous works, we show that snow saltation is characterized by two different regimes. This is not properly represented in the large scale models, which hinder the quantification of snow sublimation.
Georg Lackner, Florent Domine, Daniel F. Nadeau, Annie-Claude Parent, François Anctil, Matthieu Lafaysse, and Marie Dumont
The Cryosphere, 16, 127–142, https://doi.org/10.5194/tc-16-127-2022, https://doi.org/10.5194/tc-16-127-2022, 2022
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The surface energy budget is the sum of all incoming and outgoing energy fluxes at the Earth's surface and has a key role in the climate. We measured all these fluxes for an Arctic snowpack and found that most incoming energy from radiation is counterbalanced by thermal radiation and heat convection while sublimation was negligible. Overall, the snow model Crocus was able to simulate the observed energy fluxes well.
Abigail G. Hughes, Sonja Wahl, Tyler R. Jones, Alexandra Zuhr, Maria Hörhold, James W. C. White, and Hans Christian Steen-Larsen
The Cryosphere, 15, 4949–4974, https://doi.org/10.5194/tc-15-4949-2021, https://doi.org/10.5194/tc-15-4949-2021, 2021
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Water isotope records in Greenland and Antarctic ice cores are a valuable proxy for paleoclimate reconstruction and are traditionally thought to primarily reflect precipitation input. However,
post-depositional processes are hypothesized to contribute to the isotope climate signal. In this study we use laboratory experiments, field experiments, and modeling to show that sublimation and vapor–snow isotope exchange can rapidly influence the isotopic composition of the snowpack.
Holt Hancock, Jordy Hendrikx, Markus Eckerstorfer, and Siiri Wickström
The Cryosphere, 15, 3813–3837, https://doi.org/10.5194/tc-15-3813-2021, https://doi.org/10.5194/tc-15-3813-2021, 2021
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We investigate how snow avalanche activity in central Spitsbergen, Svalbard, is broadly controlled by atmospheric circulation. Avalanche activity in this region is generally associated with atmospheric circulation conducive to increased precipitation, wind speeds, and air temperatures near Svalbard during winter storms. Our results help place avalanche activity on Spitsbergen in the wider context of Arctic environmental change and provide a foundation for improved avalanche forecasting here.
Dimitri Osmont, Sandra Brugger, Anina Gilgen, Helga Weber, Michael Sigl, Robin L. Modini, Christoph Schwörer, Willy Tinner, Stefan Wunderle, and Margit Schwikowski
The Cryosphere, 14, 3731–3745, https://doi.org/10.5194/tc-14-3731-2020, https://doi.org/10.5194/tc-14-3731-2020, 2020
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In this interdisciplinary case study, we were able to link biomass burning emissions from the June 2017 wildfires in Portugal to their deposition in the snowpack at Jungfraujoch, Swiss Alps. We analysed black carbon and charcoal in the snowpack, calculated backward trajectories, and monitored the fire evolution by remote sensing. Such case studies help to understand the representativity of biomass burning records in ice cores and how biomass burning tracers are archived in the snowpack.
Wenkai Li, Shuzhen Hu, Pang-Chi Hsu, Weidong Guo, and Jiangfeng Wei
The Cryosphere, 14, 3565–3579, https://doi.org/10.5194/tc-14-3565-2020, https://doi.org/10.5194/tc-14-3565-2020, 2020
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Understanding the forecasting skills of the subseasonal-to-seasonal (S2S) model on Tibetan Plateau snow cover (TPSC) is the first step to applying the S2S model to hydrological forecasts over the Tibetan Plateau. This study conducted a multimodel comparison of the TPSC prediction skill to learn about their performance in capturing TPSC variability. S2S models can skillfully forecast TPSC within a lead time of 2 weeks but show limited skill beyond 3 weeks. Systematic biases of TPSC were found.
Nikolas O. Aksamit and John W. Pomeroy
The Cryosphere, 14, 2795–2807, https://doi.org/10.5194/tc-14-2795-2020, https://doi.org/10.5194/tc-14-2795-2020, 2020
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In cold regions, it is increasingly important to quantify the amount of water stored as snow at the end of winter. Current models are inconsistent in their estimates of snow sublimation due to atmospheric turbulence. Specific wind structures have been identified that amplify potential rates of surface and blowing snow sublimation during blowing snow storms. The recurrence of these motions has been modeled by a simple scaling argument that has its foundation in turbulent boundary layer theory.
Andrew J. Schwartz, Hamish A. McGowan, Alison Theobald, and Nik Callow
The Cryosphere, 14, 2755–2774, https://doi.org/10.5194/tc-14-2755-2020, https://doi.org/10.5194/tc-14-2755-2020, 2020
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This study measured energy available for snowmelt during the 2016 and 2017 snow seasons in Kosciuszko National Park, NSW, Australia, and identified common traits for days with similar weather characteristics. The analysis showed that energy available for snowmelt was highest in the days before cold fronts passed through the region due to higher air temperatures. Regardless of differences in daily weather characteristics, solar radiation contributed the highest amount of energy to snowpack melt.
Benjamin Walter, Hendrik Huwald, Josué Gehring, Yves Bühler, and Michael Lehning
The Cryosphere, 14, 1779–1794, https://doi.org/10.5194/tc-14-1779-2020, https://doi.org/10.5194/tc-14-1779-2020, 2020
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We applied a horizontally mounted low-cost precipitation radar to measure velocities, frequency of occurrence, travel distances and turbulence characteristics of blowing snow off a mountain ridge. Our analysis provides a first insight into the potential of radar measurements for determining blowing snow characteristics, improves our understanding of mountain ridge blowing snow events and serves as a valuable data basis for validating coupled numerical weather and snowpack simulations.
Charles Amory and Christoph Kittel
The Cryosphere, 13, 3405–3412, https://doi.org/10.5194/tc-13-3405-2019, https://doi.org/10.5194/tc-13-3405-2019, 2019
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Snow mass fluxes and vertical profiles of relative humidity are used to document concurrent occurrences of drifting snow and near-surface air saturation at a site dominated by katabatic winds in East Antarctica. Despite a high prevalence of drifting snow conditions, we demonstrate that saturation is reached only in the most extreme wind and transport conditions and discuss implications for the understanding of surface mass and atmospheric moisture budgets of the Antarctic ice sheet.
Varun Sharma, Louise Braud, and Michael Lehning
The Cryosphere, 13, 3239–3260, https://doi.org/10.5194/tc-13-3239-2019, https://doi.org/10.5194/tc-13-3239-2019, 2019
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Snow surfaces, under the action of wind, form beautiful shapes such as waves and dunes. This study is the first ever study to simulate these shapes using a state-of-the-art numerical modelling tool. While these beautiful and ephemeral shapes on snow surfaces are fascinating from a purely aesthetic point of view, they are also critical in regulating the transfer of heat and mass between the atmosphere and snowpacks, thus being of huge importance to the Earth system.
Yvan Orsolini, Martin Wegmann, Emanuel Dutra, Boqi Liu, Gianpaolo Balsamo, Kun Yang, Patricia de Rosnay, Congwen Zhu, Wenli Wang, Retish Senan, and Gabriele Arduini
The Cryosphere, 13, 2221–2239, https://doi.org/10.5194/tc-13-2221-2019, https://doi.org/10.5194/tc-13-2221-2019, 2019
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The Tibetan Plateau region exerts a considerable influence on regional climate, yet the snowpack over that region is poorly represented in both climate and forecast models due a large precipitation and snowfall bias. We evaluate the snowpack in state-of-the-art atmospheric reanalyses against in situ observations and satellite remote sensing products. Improved snow initialisation through better use of snow observations in reanalyses may improve medium-range to seasonal weather forecasts.
Dušan Materić, Elke Ludewig, Kangming Xu, Thomas Röckmann, and Rupert Holzinger
The Cryosphere, 13, 297–307, https://doi.org/10.5194/tc-13-297-2019, https://doi.org/10.5194/tc-13-297-2019, 2019
Niels Souverijns, Alexandra Gossart, Stef Lhermitte, Irina V. Gorodetskaya, Jacopo Grazioli, Alexis Berne, Claudio Duran-Alarcon, Brice Boudevillain, Christophe Genthon, Claudio Scarchilli, and Nicole P. M. van Lipzig
The Cryosphere, 12, 3775–3789, https://doi.org/10.5194/tc-12-3775-2018, https://doi.org/10.5194/tc-12-3775-2018, 2018
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Snowfall observations over Antarctica are scarce and currently limited to information from the CloudSat satellite. Here, a first evaluation of the CloudSat snowfall record is performed using observations of ground-based precipitation radars. Results indicate an accurate representation of the snowfall climatology over Antarctica, despite the low overpass frequency of the satellite, outperforming state-of-the-art model estimates. Individual snowfall events are however not well represented.
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Short summary
Chemical reactions in sea salt embedded in coastal polar snow impact the composition and air quality of the atmosphere. Here, we investigate the phase changes of sodium chloride. This is of importance as chemical reactions proceed faster in liquid solutions compared to in solid salt and the precise precipitation temperature of sodium chloride is still under debate. We focus on the upper nanometres of sodium chloride–ice samples because of their role as a reactive interface in the environment.
Chemical reactions in sea salt embedded in coastal polar snow impact the composition and air...
