Articles | Volume 17, issue 7
https://doi.org/10.5194/tc-17-2909-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/tc-17-2909-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Black carbon concentrations and modeled smoke deposition fluxes to the bare-ice dark zone of the Greenland Ice Sheet
Department of Environmental Sciences, Western Washington University, WA, USA
Peng Xian
Aerosol and Radiation Section of the Marine Meteorology Division, Naval Research Laboratory, Monterey, California, USA
Joshua P. Schwarz
Chemical Sciences Laboratory, NOAA Earth System Research Laboratories (ESRL), Boulder, CO, USA
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Alia L. Khan, Heidi M. Dierssen, Ted A. Scambos, Juan Höfer, and Raul R. Cordero
The Cryosphere, 15, 133–148, https://doi.org/10.5194/tc-15-133-2021, https://doi.org/10.5194/tc-15-133-2021, 2021
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We present radiative forcing (RF) estimates by snow algae in the Antarctic Peninsula (AP) region from multi-year measurements of solar radiation and ground-based hyperspectral characterization of red and green snow algae collected during a brief field expedition in austral summer 2018. Mean daily RF was double for green (~26 W m−2) vs. red (~13 W m−2) snow algae during the peak growing season, which is on par with midlatitude dust attributions capable of advancing snowmelt.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024, https://doi.org/10.5194/acp-24-10985-2024, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) from the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign. This study reveals the compositions, abundance, sizes, and mixing states of TBs and shows that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass-burning events and ages, enhancing our knowledge of TB emissions and our understanding of their climate impact.
Kira Zeider, Grace Betito, Anthony Bucholtz, Peng Xian, Annette Walker, and Armin Sorooshian
Atmos. Chem. Phys., 24, 9059–9083, https://doi.org/10.5194/acp-24-9059-2024, https://doi.org/10.5194/acp-24-9059-2024, 2024
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The predominant wind direction along the California coast (northerly) reverses several times during the summer (to southerly). The effects of these wind reversals on aerosol and cloud characteristics are not well understood. Using data from multiple datasets we found that southerly flow periods had enhanced signatures of anthropogenic emissions due to shipping and continental sources, and clouds had more but smaller droplets.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Georgios I. Gkatzelis, Matthew M. Coggon, Chelsea E. Stockwell, Rebecca S. Hornbrook, Hannah Allen, Eric C. Apel, Megan M. Bela, Donald R. Blake, Ilann Bourgeois, Steven S. Brown, Pedro Campuzano-Jost, Jason M. St. Clair, James H. Crawford, John D. Crounse, Douglas A. Day, Joshua P. DiGangi, Glenn S. Diskin, Alan Fried, Jessica B. Gilman, Hongyu Guo, Johnathan W. Hair, Hannah S. Halliday, Thomas F. Hanisco, Reem Hannun, Alan Hills, L. Gregory Huey, Jose L. Jimenez, Joseph M. Katich, Aaron Lamplugh, Young Ro Lee, Jin Liao, Jakob Lindaas, Stuart A. McKeen, Tomas Mikoviny, Benjamin A. Nault, J. Andrew Neuman, John B. Nowak, Demetrios Pagonis, Jeff Peischl, Anne E. Perring, Felix Piel, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Thomas B. Ryerson, Melinda K. Schueneman, Rebecca H. Schwantes, Joshua P. Schwarz, Kanako Sekimoto, Vanessa Selimovic, Taylor Shingler, David J. Tanner, Laura Tomsche, Krystal T. Vasquez, Patrick R. Veres, Rebecca Washenfelder, Petter Weibring, Paul O. Wennberg, Armin Wisthaler, Glenn M. Wolfe, Caroline C. Womack, Lu Xu, Katherine Ball, Robert J. Yokelson, and Carsten Warneke
Atmos. Chem. Phys., 24, 929–956, https://doi.org/10.5194/acp-24-929-2024, https://doi.org/10.5194/acp-24-929-2024, 2024
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This study reports emissions of gases and particles from wildfires. These emissions are related to chemical proxies that can be measured by satellite and incorporated into models to improve predictions of wildfire impacts on air quality and climate.
Blake T. Sorenson, Jianglong Zhang, Jeffrey S. Reid, Peng Xian, and Shawn L. Jaker
Atmos. Chem. Phys., 23, 7161–7175, https://doi.org/10.5194/acp-23-7161-2023, https://doi.org/10.5194/acp-23-7161-2023, 2023
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We quality-control Ozone Monitoring Instrument (OMI) aerosol index data by identifying row anomalies and removing systematic biases, using the data to quantify trends in UV-absorbing aerosols over the Arctic region. We found decreasing trends in UV-absorbing aerosols in spring months and increasing trends in summer months. For the first time, observational evidence of increasing trends in UV-absorbing aerosols over the North Pole is found using the OMI data, especially over the last half decade.
Haihui Zhu, Randall V. Martin, Betty Croft, Shixian Zhai, Chi Li, Liam Bindle, Jeffrey R. Pierce, Rachel Y.-W. Chang, Bruce E. Anderson, Luke D. Ziemba, Johnathan W. Hair, Richard A. Ferrare, Chris A. Hostetler, Inderjeet Singh, Deepangsu Chatterjee, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jack E. Dibb, Joshua S. Schwarz, and Andrew Weinheimer
Atmos. Chem. Phys., 23, 5023–5042, https://doi.org/10.5194/acp-23-5023-2023, https://doi.org/10.5194/acp-23-5023-2023, 2023
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Particle size of atmospheric aerosol is important for estimating its climate and health effects, but simulating atmospheric aerosol size is computationally demanding. This study derives a simple parameterization of the size of organic and secondary inorganic ambient aerosol that can be applied to atmospheric models. Applying this parameterization allows a better representation of the global spatial pattern of aerosol size, as verified by ground and airborne measurements.
Juli I. Rubin, Jeffrey S. Reid, Peng Xian, Christopher M. Selman, and Thomas F. Eck
Atmos. Chem. Phys., 23, 4059–4090, https://doi.org/10.5194/acp-23-4059-2023, https://doi.org/10.5194/acp-23-4059-2023, 2023
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This work aims to quantify the covariability between aerosol optical depth/extinction with water vapor (PW) globally, using NASA AERONET observations and NAAPS model data. Findings are important for data assimilation and radiative transfer. The study shows statistically significant and positive AOD–PW relationships are found across the globe, varying in strength with location and season and tied to large-scale aerosol events. Hygroscopic growth was also found to be an important factor.
Youhua Tang, Patrick C. Campbell, Pius Lee, Rick Saylor, Fanglin Yang, Barry Baker, Daniel Tong, Ariel Stein, Jianping Huang, Ho-Chun Huang, Li Pan, Jeff McQueen, Ivanka Stajner, Jose Tirado-Delgado, Youngsun Jung, Melissa Yang, Ilann Bourgeois, Jeff Peischl, Tom Ryerson, Donald Blake, Joshua Schwarz, Jose-Luis Jimenez, James Crawford, Glenn Diskin, Richard Moore, Johnathan Hair, Greg Huey, Andrew Rollins, Jack Dibb, and Xiaoyang Zhang
Geosci. Model Dev., 15, 7977–7999, https://doi.org/10.5194/gmd-15-7977-2022, https://doi.org/10.5194/gmd-15-7977-2022, 2022
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This paper compares two meteorological datasets for driving a regional air quality model: a regional meteorological model using WRF (WRF-CMAQ) and direct interpolation from an operational global model (GFS-CMAQ). In the comparison with surface measurements and aircraft data in summer 2019, these two methods show mixed performance depending on the corresponding meteorological settings. Direct interpolation is found to be a viable method to drive air quality models.
Eva-Lou Edwards, Jeffrey S. Reid, Peng Xian, Sharon P. Burton, Anthony L. Cook, Ewan C. Crosbie, Marta A. Fenn, Richard A. Ferrare, Sean W. Freeman, John W. Hair, David B. Harper, Chris A. Hostetler, Claire E. Robinson, Amy Jo Scarino, Michael A. Shook, G. Alexander Sokolowsky, Susan C. van den Heever, Edward L. Winstead, Sarah Woods, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 12961–12983, https://doi.org/10.5194/acp-22-12961-2022, https://doi.org/10.5194/acp-22-12961-2022, 2022
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This study compares NAAPS-RA model simulations of aerosol optical thickness (AOT) and extinction to those retrieved with a high spectral resolution lidar near the Philippines. Agreement for AOT was good, and extinction agreement was strongest below 1500 m. Substituting dropsonde relative humidities into NAAPS-RA did not drastically improve agreement, and we discuss potential reasons why. Accurately modeling future conditions in this region is crucial due to its susceptibility to climate change.
Aditya Kumar, R. Bradley Pierce, Ravan Ahmadov, Gabriel Pereira, Saulo Freitas, Georg Grell, Chris Schmidt, Allen Lenzen, Joshua P. Schwarz, Anne E. Perring, Joseph M. Katich, John Hair, Jose L. Jimenez, Pedro Campuzano-Jost, and Hongyu Guo
Atmos. Chem. Phys., 22, 10195–10219, https://doi.org/10.5194/acp-22-10195-2022, https://doi.org/10.5194/acp-22-10195-2022, 2022
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We use the WRF-Chem model with new implementations of GOES-16 wildfire emissions and plume rise based on fire radiative power (FRP) to interpret aerosol observations during the 2019 NASA–NOAA FIREX-AQ field campaign and perform model evaluations. The model shows significant improvements in simulating the variety of aerosol loading environments sampled during FIREX-AQ. Our results also highlight the importance of accurate wildfire diurnal cycle and aerosol chemical mechanisms in models.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Linghan Zeng, Jack Dibb, Eric Scheuer, Joseph M. Katich, Joshua P. Schwarz, Ilann Bourgeois, Jeff Peischl, Tom Ryerson, Carsten Warneke, Anne E. Perring, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Richard H. Moore, Elizabeth B. Wiggins, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Lu Xu, and Rodney J. Weber
Atmos. Chem. Phys., 22, 8009–8036, https://doi.org/10.5194/acp-22-8009-2022, https://doi.org/10.5194/acp-22-8009-2022, 2022
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Wildfires emit aerosol particles containing brown carbon material that affects visibility and global climate and is toxic. Brown carbon is poorly characterized due to measurement limitations, and its evolution in the atmosphere is not well known. We report on aircraft measurements of brown carbon from large wildfires in the western United States. We compare two methods for measuring brown carbon and study the evolution of brown carbon in the smoke as it moved away from the burning regions.
Joseph S. Schlosser, Connor Stahl, Armin Sorooshian, Yen Thi-Hoang Le, Ki-Joon Jeon, Peng Xian, Carolyn E. Jordan, Katherine R. Travis, James H. Crawford, Sung Yong Gong, Hye-Jung Shin, In-Ho Song, and Jong-sang Youn
Atmos. Chem. Phys., 22, 7505–7522, https://doi.org/10.5194/acp-22-7505-2022, https://doi.org/10.5194/acp-22-7505-2022, 2022
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During a major haze pollution episode in March 2019, anthropogenic emissions were dominant in the boundary layer over Incheon and Seoul, South Korea. Using supermicrometer and submicrometer size- and chemistry-resolved aerosol particle measurements taken during this haze pollution period, this work shows that local emissions and a shallow boundary layer, enhanced humidity, and low temperature promoted local heterogeneous formation of secondary inorganic and organic aerosol species.
Meloë S. F. Kacenelenbogen, Qian Tan, Sharon P. Burton, Otto P. Hasekamp, Karl D. Froyd, Yohei Shinozuka, Andreas J. Beyersdorf, Luke Ziemba, Kenneth L. Thornhill, Jack E. Dibb, Taylor Shingler, Armin Sorooshian, Reed W. Espinosa, Vanderlei Martins, Jose L. Jimenez, Pedro Campuzano-Jost, Joshua P. Schwarz, Matthew S. Johnson, Jens Redemann, and Gregory L. Schuster
Atmos. Chem. Phys., 22, 3713–3742, https://doi.org/10.5194/acp-22-3713-2022, https://doi.org/10.5194/acp-22-3713-2022, 2022
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The impact of aerosols on Earth's radiation budget and human health is important and strongly depends on their composition. One desire of our scientific community is to derive the composition of the aerosol from satellite sensors. However, satellites observe aerosol optical properties (and not aerosol composition) based on remote sensing instrumentation. This study assesses how much aerosol optical properties can tell us about aerosol composition.
Charles A. Brock, Karl D. Froyd, Maximilian Dollner, Christina J. Williamson, Gregory Schill, Daniel M. Murphy, Nicholas J. Wagner, Agnieszka Kupc, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jason C. Schroder, Douglas A. Day, Derek J. Price, Bernadett Weinzierl, Joshua P. Schwarz, Joseph M. Katich, Siyuan Wang, Linghan Zeng, Rodney Weber, Jack Dibb, Eric Scheuer, Glenn S. Diskin, Joshua P. DiGangi, ThaoPaul Bui, Jonathan M. Dean-Day, Chelsea R. Thompson, Jeff Peischl, Thomas B. Ryerson, Ilann Bourgeois, Bruce C. Daube, Róisín Commane, and Steven C. Wofsy
Atmos. Chem. Phys., 21, 15023–15063, https://doi.org/10.5194/acp-21-15023-2021, https://doi.org/10.5194/acp-21-15023-2021, 2021
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The Atmospheric Tomography Mission was an airborne study that mapped the chemical composition of the remote atmosphere. From this, we developed a comprehensive description of aerosol properties that provides a unique, global-scale dataset against which models can be compared. The data show the polluted nature of the remote atmosphere in the Northern Hemisphere and quantify the contributions of sea salt, dust, soot, biomass burning particles, and pollution particles to the haziness of the sky.
Marco Zanatta, Andreas Herber, Zsófia Jurányi, Oliver Eppers, Johannes Schneider, and Joshua P. Schwarz
Atmos. Chem. Phys., 21, 9329–9342, https://doi.org/10.5194/acp-21-9329-2021, https://doi.org/10.5194/acp-21-9329-2021, 2021
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Saline snow samples were collected from the sea ice in the Fram Strait. Laboratory experiments revealed that sea salt can bias the quantification of black carbon with a laser-induced incandescence technique. The maximum underestimation was quantified to reach values of 80 %–90 %. This salt-induced interference is reported here for the first time and should be considered in future studies aiming to quantify black carbon in snow in marine environments.
Caroline C. Womack, Katherine M. Manfred, Nicholas L. Wagner, Gabriela Adler, Alessandro Franchin, Kara D. Lamb, Ann M. Middlebrook, Joshua P. Schwarz, Charles A. Brock, Steven S. Brown, and Rebecca A. Washenfelder
Atmos. Chem. Phys., 21, 7235–7252, https://doi.org/10.5194/acp-21-7235-2021, https://doi.org/10.5194/acp-21-7235-2021, 2021
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Microscopic particles interact with sunlight and affect the earth's climate in ways that are not fully understood. Aerosols from wildfire smoke present particular challenges due to their complexity in shape and composition. We demonstrate that we can experimentally measure aerosol optical properties for many types of smoke particles, using measurements of smoke from controlled burns, but that the method does not work well for smoke with high soot content.
Alia L. Khan, Heidi M. Dierssen, Ted A. Scambos, Juan Höfer, and Raul R. Cordero
The Cryosphere, 15, 133–148, https://doi.org/10.5194/tc-15-133-2021, https://doi.org/10.5194/tc-15-133-2021, 2021
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We present radiative forcing (RF) estimates by snow algae in the Antarctic Peninsula (AP) region from multi-year measurements of solar radiation and ground-based hyperspectral characterization of red and green snow algae collected during a brief field expedition in austral summer 2018. Mean daily RF was double for green (~26 W m−2) vs. red (~13 W m−2) snow algae during the peak growing season, which is on par with midlatitude dust attributions capable of advancing snowmelt.
Jianglong Zhang, Robert J. D. Spurr, Jeffrey S. Reid, Peng Xian, Peter R. Colarco, James R. Campbell, Edward J. Hyer, and Nancy L. Baker
Geosci. Model Dev., 14, 27–42, https://doi.org/10.5194/gmd-14-27-2021, https://doi.org/10.5194/gmd-14-27-2021, 2021
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A first-of-its-kind scheme has been developed for assimilating Ozone Monitoring Instrument (OMI) aerosol index (AI) measurements into the Naval Aerosol Analysis and Predictive System. Improvements in model simulations demonstrate the utility of OMI AI data assimilation for improving the accuracy of aerosol model analysis over cloudy regions and bright surfaces. This study can be considered one of the first attempts at direct radiance assimilation in the UV spectrum for aerosol analyses.
Peng Xian, Philip J. Klotzbach, Jason P. Dunion, Matthew A. Janiga, Jeffrey S. Reid, Peter R. Colarco, and Zak Kipling
Atmos. Chem. Phys., 20, 15357–15378, https://doi.org/10.5194/acp-20-15357-2020, https://doi.org/10.5194/acp-20-15357-2020, 2020
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Using dust AOD (DAOD) data from three aerosol reanalyses, we explored the correlative relationships between DAOD and multiple indices representing seasonal Atlantic TC activities. A robust negative correlation with Caribbean DAOD and Atlantic TC activity was found. We documented for the first time the regional differences of this relationship for over the Caribbean and the tropical North Atlantic. We also evaluated the impacts of potential confounding climate factors in this relationship.
Steven Albers, Stephen M. Saleeby, Sonia Kreidenweis, Qijing Bian, Peng Xian, Zoltan Toth, Ravan Ahmadov, Eric James, and Steven D. Miller
Atmos. Meas. Tech., 13, 3235–3261, https://doi.org/10.5194/amt-13-3235-2020, https://doi.org/10.5194/amt-13-3235-2020, 2020
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A fast 3D visible-light forward operator is used to realistically visualize, validate, and potentially assimilate ground- and space-based camera and satellite imagery with NWP models. Three-dimensional fields of hydrometeors, aerosols, and 2D land surface variables are considered in the generation of radiance fields and RGB imagery from a variety of vantage points.
Pablo E. Saide, Meng Gao, Zifeng Lu, Daniel L. Goldberg, David G. Streets, Jung-Hun Woo, Andreas Beyersdorf, Chelsea A. Corr, Kenneth L. Thornhill, Bruce Anderson, Johnathan W. Hair, Amin R. Nehrir, Glenn S. Diskin, Jose L. Jimenez, Benjamin A. Nault, Pedro Campuzano-Jost, Jack Dibb, Eric Heim, Kara D. Lamb, Joshua P. Schwarz, Anne E. Perring, Jhoon Kim, Myungje Choi, Brent Holben, Gabriele Pfister, Alma Hodzic, Gregory R. Carmichael, Louisa Emmons, and James H. Crawford
Atmos. Chem. Phys., 20, 6455–6478, https://doi.org/10.5194/acp-20-6455-2020, https://doi.org/10.5194/acp-20-6455-2020, 2020
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Air quality forecasts over the Korean Peninsula captured aerosol optical depth but largely overpredicted surface PM during a Chinese haze transport event. Model deficiency was related to the calculation of optical properties. In order to improve it, aerosol size representation needs to be refined in the calculations, and the representation of aerosol properties, such as size distribution, chemical composition, refractive index, hygroscopicity parameter, and density, needs to be improved.
Alma Hodzic, Pedro Campuzano-Jost, Huisheng Bian, Mian Chin, Peter R. Colarco, Douglas A. Day, Karl D. Froyd, Bernd Heinold, Duseong S. Jo, Joseph M. Katich, John K. Kodros, Benjamin A. Nault, Jeffrey R. Pierce, Eric Ray, Jacob Schacht, Gregory P. Schill, Jason C. Schroder, Joshua P. Schwarz, Donna T. Sueper, Ina Tegen, Simone Tilmes, Kostas Tsigaridis, Pengfei Yu, and Jose L. Jimenez
Atmos. Chem. Phys., 20, 4607–4635, https://doi.org/10.5194/acp-20-4607-2020, https://doi.org/10.5194/acp-20-4607-2020, 2020
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Organic aerosol (OA) is a key source of uncertainty in aerosol climate effects. We present the first pole-to-pole OA characterization during the NASA Atmospheric Tomography aircraft mission. OA has a strong seasonal and zonal variability, with the highest levels in summer and over fire-influenced regions and the lowest ones in the southern high latitudes. We show that global models predict the OA distribution well but not the relative contribution of OA emissions vs. chemical production.
Therese S. Carter, Colette L. Heald, Jose L. Jimenez, Pedro Campuzano-Jost, Yutaka Kondo, Nobuhiro Moteki, Joshua P. Schwarz, Christine Wiedinmyer, Anton S. Darmenov, Arlindo M. da Silva, and Johannes W. Kaiser
Atmos. Chem. Phys., 20, 2073–2097, https://doi.org/10.5194/acp-20-2073-2020, https://doi.org/10.5194/acp-20-2073-2020, 2020
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Fires and the smoke they emit impact air quality, health, and climate, but the abundance and properties of smoke remain uncertain and poorly constrained. To explore this, we compare model simulations driven by four commonly-used fire emission inventories with surface, aloft, and satellite observations. We show that across inventories smoke emissions differ by factors of 4 to 7 over North America, challenging our ability to accurately characterize the impact of smoke on air quality and climate.
Miguel Ricardo A. Hilario, Melliza T. Cruz, Maria Obiminda L. Cambaliza, Jeffrey S. Reid, Peng Xian, James B. Simpas, Nofel D. Lagrosas, Sherdon Niño Y. Uy, Steve Cliff, and Yongjing Zhao
Atmos. Chem. Phys., 20, 1255–1276, https://doi.org/10.5194/acp-20-1255-2020, https://doi.org/10.5194/acp-20-1255-2020, 2020
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The research apportions size-resolved aerosol contributions from the South China Sea during the Vasco research cruise in September 2011. As aerosols can affect precipitation rates and cloud formation, identifying sources is key to characterizing the region and developing our understanding of aerosol–cloud behavior. A strong biomass burning signal was identified using elemental particulate matter in the fine and ultrafine size ranges. Oil combustion, soil dust, and sea spray were also identified.
Charles A. Brock, Christina Williamson, Agnieszka Kupc, Karl D. Froyd, Frank Erdesz, Nicholas Wagner, Matthews Richardson, Joshua P. Schwarz, Ru-Shan Gao, Joseph M. Katich, Pedro Campuzano-Jost, Benjamin A. Nault, Jason C. Schroder, Jose L. Jimenez, Bernadett Weinzierl, Maximilian Dollner, ThaoPaul Bui, and Daniel M. Murphy
Atmos. Meas. Tech., 12, 3081–3099, https://doi.org/10.5194/amt-12-3081-2019, https://doi.org/10.5194/amt-12-3081-2019, 2019
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From 2016 to 2018 a NASA aircraft profiled the atmosphere from 180 m to ~12 km from the Arctic to the Antarctic over both the Pacific and Atlantic oceans. This program, ATom, sought to sample atmospheric chemical composition to compare with global climate models. We describe the how measurements of particulate matter were made during ATom, and show that the instrument performance was excellent. Data from this project can be used with confidence to evaluate models and compare with satellites.
J. Christopher Kaiser, Johannes Hendricks, Mattia Righi, Patrick Jöckel, Holger Tost, Konrad Kandler, Bernadett Weinzierl, Daniel Sauer, Katharina Heimerl, Joshua P. Schwarz, Anne E. Perring, and Thomas Popp
Geosci. Model Dev., 12, 541–579, https://doi.org/10.5194/gmd-12-541-2019, https://doi.org/10.5194/gmd-12-541-2019, 2019
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The implementation of the aerosol microphysics submodel MADE3 into the global atmospheric chemistry model EMAC is described and evaluated against an extensive pool of observational data, focusing on aerosol mass and number concentrations, size distributions, composition, and optical properties. EMAC (MADE3) is able to reproduce main aerosol properties reasonably well, in line with the performance of other global aerosol models.
Mayra I. Oyola, James R. Campbell, Peng Xian, Anthony Bucholtz, Richard A. Ferrare, Sharon P. Burton, Olga Kalashnikova, Benjamin C. Ruston, and Simone Lolli
Atmos. Chem. Phys., 19, 205–218, https://doi.org/10.5194/acp-19-205-2019, https://doi.org/10.5194/acp-19-205-2019, 2019
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We conceptualized the aerosol radiative impact of an inline aerosol analysis field coupled with a global meteorological forecast system utilizing NAAPS and NAVGEM analysis and surface albedo fields. Model simulations were compared with in situ validation data collected during the NASA 2013 SEAC4RS experiment. Instantaneous heating rates peaked around 7 K day-1 in the lower part of the troposphere, while the HSRL profiles resulted in values of up to 18 K day-1 in the in the mid-troposphere.
Alexa D. Ross, Robert E. Holz, Gregory Quinn, Jeffrey S. Reid, Peng Xian, F. Joseph Turk, and Derek J. Posselt
Atmos. Chem. Phys., 18, 12747–12764, https://doi.org/10.5194/acp-18-12747-2018, https://doi.org/10.5194/acp-18-12747-2018, 2018
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This paper explores how clouds and aerosols interact over Southeast Asia. We introduce a new collocated dataset called the Curtain Cloud-Aerosol Regional A-Train (CCARA) product. CCARA is special because it combines satellite observations with model reanalysis. We find that increased aerosol corresponds to smaller observed liquid cloud droplets in some areas. Other areas experienced little to no change in effective radius (droplet size) when aerosol amount increased.
Katherine M. Manfred, Rebecca A. Washenfelder, Nicholas L. Wagner, Gabriela Adler, Frank Erdesz, Caroline C. Womack, Kara D. Lamb, Joshua P. Schwarz, Alessandro Franchin, Vanessa Selimovic, Robert J. Yokelson, and Daniel M. Murphy
Atmos. Chem. Phys., 18, 1879–1894, https://doi.org/10.5194/acp-18-1879-2018, https://doi.org/10.5194/acp-18-1879-2018, 2018
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In this study, we use a new laser imaging nephelometer to measure the bulk aerosol scattering phase function for biomass burning aerosol from controlled fires. By comparing measurements to models for spherical and fractal particles, we demonstrate that the dominant morphology varies by fuel type. This instrument has unique capabilities to directly measure how morphology affects optical properties, and can be used in the future for important validations of remote sensing retrievals.
Xuan Wang, Colette L. Heald, Jiumeng Liu, Rodney J. Weber, Pedro Campuzano-Jost, Jose L. Jimenez, Joshua P. Schwarz, and Anne E. Perring
Atmos. Chem. Phys., 18, 635–653, https://doi.org/10.5194/acp-18-635-2018, https://doi.org/10.5194/acp-18-635-2018, 2018
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Brown carbon (BrC) contributes significantly to uncertainty in estimating the global direct radiative effect (DRE) of aerosols. We develop a global model simulation of BrC and test it against BrC absorption measurements from two aircraft campaigns in the continental United States. We suggest that BrC DRE has been overestimated previously due to the lack of observational constraints from direct measurements and omission of the effects of photochemical whitening.
Ellis Shipley Robinson, Ru-Shan Gao, Joshua P. Schwarz, David W. Fahey, and Anne E. Perring
Atmos. Meas. Tech., 10, 1755–1768, https://doi.org/10.5194/amt-10-1755-2017, https://doi.org/10.5194/amt-10-1755-2017, 2017
Samuel A. Atwood, Jeffrey S. Reid, Sonia M. Kreidenweis, Donald R. Blake, Haflidi H. Jonsson, Nofel D. Lagrosas, Peng Xian, Elizabeth A. Reid, Walter R. Sessions, and James B. Simpas
Atmos. Chem. Phys., 17, 1105–1123, https://doi.org/10.5194/acp-17-1105-2017, https://doi.org/10.5194/acp-17-1105-2017, 2017
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Aerosol particles were measured by ship in remote marine regions of the South China Sea as part of the 2012 7 Southeast Asian Studies (7SEAS) experiments. As the particle populations changed throughout the experiment, the distribution of particle sizes and the amount of water that collected on them changed as well. These changes were associated with various impacts from smoke, sea salt, and pollution sources, and impact how clouds form and precipitation occurs in the region.
Jeffrey S. Reid, Peng Xian, Brent N. Holben, Edward J. Hyer, Elizabeth A. Reid, Santo V. Salinas, Jianglong Zhang, James R. Campbell, Boon Ning Chew, Robert E. Holz, Arunas P. Kuciauskas, Nofel Lagrosas, Derek J. Posselt, Charles R. Sampson, Annette L. Walker, E. Judd Welton, and Chidong Zhang
Atmos. Chem. Phys., 16, 14041–14056, https://doi.org/10.5194/acp-16-14041-2016, https://doi.org/10.5194/acp-16-14041-2016, 2016
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This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
Jeffrey S. Reid, Nofel D. Lagrosas, Haflidi H. Jonsson, Elizabeth A. Reid, Samuel A. Atwood, Thomas J. Boyd, Virendra P. Ghate, Peng Xian, Derek J. Posselt, James B. Simpas, Sherdon N. Uy, Kimo Zaiger, Donald R. Blake, Anthony Bucholtz, James R. Campbell, Boon Ning Chew, Steven S. Cliff, Brent N. Holben, Robert E. Holz, Edward J. Hyer, Sonia M. Kreidenweis, Arunas P. Kuciauskas, Simone Lolli, Min Oo, Kevin D. Perry, Santo V. Salinas, Walter R. Sessions, Alexander Smirnov, Annette L. Walker, Qing Wang, Liya Yu, Jianglong Zhang, and Yongjing Zhao
Atmos. Chem. Phys., 16, 14057–14078, https://doi.org/10.5194/acp-16-14057-2016, https://doi.org/10.5194/acp-16-14057-2016, 2016
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This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
Carsten Warneke, Michael Trainer, Joost A. de Gouw, David D. Parrish, David W. Fahey, A. R. Ravishankara, Ann M. Middlebrook, Charles A. Brock, James M. Roberts, Steven S. Brown, Jonathan A. Neuman, Brian M. Lerner, Daniel Lack, Daniel Law, Gerhard Hübler, Iliana Pollack, Steven Sjostedt, Thomas B. Ryerson, Jessica B. Gilman, Jin Liao, John Holloway, Jeff Peischl, John B. Nowak, Kenneth C. Aikin, Kyung-Eun Min, Rebecca A. Washenfelder, Martin G. Graus, Mathew Richardson, Milos Z. Markovic, Nick L. Wagner, André Welti, Patrick R. Veres, Peter Edwards, Joshua P. Schwarz, Timothy Gordon, William P. Dube, Stuart A. McKeen, Jerome Brioude, Ravan Ahmadov, Aikaterini Bougiatioti, Jack J. Lin, Athanasios Nenes, Glenn M. Wolfe, Thomas F. Hanisco, Ben H. Lee, Felipe D. Lopez-Hilfiker, Joel A. Thornton, Frank N. Keutsch, Jennifer Kaiser, Jingqiu Mao, and Courtney D. Hatch
Atmos. Meas. Tech., 9, 3063–3093, https://doi.org/10.5194/amt-9-3063-2016, https://doi.org/10.5194/amt-9-3063-2016, 2016
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In this paper we describe the experimental approach, the science goals and early results of the NOAA SENEX campaign, which was focused on studying the interactions between biogenic and anthropogenic emissions to form secondary pollutants.
During SENEX, the NOAA WP-3D aircraft conducted 20 research flights between 27 May and 10 July 2013 based out of Smyrna, TN. The SENEX flights included day- and nighttime flights in the Southeast as well as flights over areas with intense shale gas extraction.
Charles A. Brock, Nicholas L. Wagner, Bruce E. Anderson, Alexis R. Attwood, Andreas Beyersdorf, Pedro Campuzano-Jost, Annmarie G. Carlton, Douglas A. Day, Glenn S. Diskin, Timothy D. Gordon, Jose L. Jimenez, Daniel A. Lack, Jin Liao, Milos Z. Markovic, Ann M. Middlebrook, Nga L. Ng, Anne E. Perring, Matthews S. Richardson, Joshua P. Schwarz, Rebecca A. Washenfelder, Andre Welti, Lu Xu, Luke D. Ziemba, and Daniel M. Murphy
Atmos. Chem. Phys., 16, 4987–5007, https://doi.org/10.5194/acp-16-4987-2016, https://doi.org/10.5194/acp-16-4987-2016, 2016
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Microscopic pollution particles make the atmosphere look hazy and also cool the earth by sending sunlight back to space. When the air is moist, these particles swell with water and scatter even more sunlight. We showed that particles formed from organic material – which dominates particulate pollution in the southeastern U.S. – does not take up water very effectively, toward the low end of most previous studies. We also found a better way to mathematically describe this swelling process.
Charles A. Brock, Nicholas L. Wagner, Bruce E. Anderson, Andreas Beyersdorf, Pedro Campuzano-Jost, Douglas A. Day, Glenn S. Diskin, Timothy D. Gordon, Jose L. Jimenez, Daniel A. Lack, Jin Liao, Milos Z. Markovic, Ann M. Middlebrook, Anne E. Perring, Matthews S. Richardson, Joshua P. Schwarz, Andre Welti, Luke D. Ziemba, and Daniel M. Murphy
Atmos. Chem. Phys., 16, 5009–5019, https://doi.org/10.5194/acp-16-5009-2016, https://doi.org/10.5194/acp-16-5009-2016, 2016
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Two research aircraft made dozens of vertical profiles over rural areas in the southeastern US in summer 2013. These measurements show that, in addition to how much pollution was present and how moist the atmosphere was, the size of the pollutant particles affected how much sunlight was reflected back to space. These measurements will help climate modelers determine which characteristics of pollution are important to predict with accuracy.
Peng Lynch, Jeffrey S. Reid, Douglas L. Westphal, Jianglong Zhang, Timothy F. Hogan, Edward J. Hyer, Cynthia A. Curtis, Dean A. Hegg, Yingxi Shi, James R. Campbell, Juli I. Rubin, Walter R. Sessions, F. Joseph Turk, and Annette L. Walker
Geosci. Model Dev., 9, 1489–1522, https://doi.org/10.5194/gmd-9-1489-2016, https://doi.org/10.5194/gmd-9-1489-2016, 2016
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An 11-year, 1-degree aerosol reanalysis is presented for use in studies of aerosol effects on climate and atmospheric processes. The reanalysis uses the Navy Aerosol Analysis and Prediction System, constrained by aerosol optical thickness (AOT) data from NASA sensors. Fine and coarse mode AOT at 550 nm agrees well with ground-based measurements, and reproduces the decadal AOT trends found using standalone satellite products. This dataset is a resource for basic and applied science research.
Juli I. Rubin, Jeffrey S. Reid, James A. Hansen, Jeffrey L. Anderson, Nancy Collins, Timothy J. Hoar, Timothy Hogan, Peng Lynch, Justin McLay, Carolyn A. Reynolds, Walter R. Sessions, Douglas L. Westphal, and Jianglong Zhang
Atmos. Chem. Phys., 16, 3927–3951, https://doi.org/10.5194/acp-16-3927-2016, https://doi.org/10.5194/acp-16-3927-2016, 2016
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This work tests the use of an ensemble prediction system for aerosol forecasting, including an ensemble adjustment Kalman filter for MODIS AOT assimilation. Key findings include (1) meteorology and source-perturbed ensembles are needed to capture long-range transport and near-source aerosol events, (2) adaptive covariance inflation is recommended for assimilating spatially heterogeneous observations and (3) the ensemble system captures sharp gradients relative to a deterministic/variational system.
Cenlin He, Qinbin Li, Kuo-Nan Liou, Ling Qi, Shu Tao, and Joshua P. Schwarz
Atmos. Chem. Phys., 16, 3077–3098, https://doi.org/10.5194/acp-16-3077-2016, https://doi.org/10.5194/acp-16-3077-2016, 2016
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Blarck carbon aging significantly affects its global distribution and thus climatic effects. This study develops a microphysics-based BC aging scheme in a global model, which substantially improves model simulations of BC over the remote Pacific. The microphysical scheme shows fast aging over source regions and much slower aging in remote regions. The microphysical aging significantly reduces global BC burden and lifetime, showing important implications for the estimate of BC radiative effects.
P. S. Kim, D. J. Jacob, J. A. Fisher, K. Travis, K. Yu, L. Zhu, R. M. Yantosca, M. P. Sulprizio, J. L. Jimenez, P. Campuzano-Jost, K. D. Froyd, J. Liao, J. W. Hair, M. A. Fenn, C. F. Butler, N. L. Wagner, T. D. Gordon, A. Welti, P. O. Wennberg, J. D. Crounse, J. M. St. Clair, A. P. Teng, D. B. Millet, J. P. Schwarz, M. Z. Markovic, and A. E. Perring
Atmos. Chem. Phys., 15, 10411–10433, https://doi.org/10.5194/acp-15-10411-2015, https://doi.org/10.5194/acp-15-10411-2015, 2015
J. Liu, E. Scheuer, J. Dibb, G. S. Diskin, L. D. Ziemba, K. L. Thornhill, B. E. Anderson, A. Wisthaler, T. Mikoviny, J. J. Devi, M. Bergin, A. E. Perring, M. Z. Markovic, J. P. Schwarz, P. Campuzano-Jost, D. A. Day, J. L. Jimenez, and R. J. Weber
Atmos. Chem. Phys., 15, 7841–7858, https://doi.org/10.5194/acp-15-7841-2015, https://doi.org/10.5194/acp-15-7841-2015, 2015
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Brown carbon (BrC) is found throughout the US continental troposphere during a summer of extensive biomass burning and its prevalence relative to black carbon (BC) increases with altitude. A radiative transfer model based on direct measurements of aerosol scattering and absorption by BC and BrC shows BrC reduces top-of-atmosphere forcing by 20%. A method to estimate BrC radiative forcing efficiencies from surface-based measurements is provided.
N. L. Wagner, C. A. Brock, W. M. Angevine, A. Beyersdorf, P. Campuzano-Jost, D. Day, J. A. de Gouw, G. S. Diskin, T. D. Gordon, M. G. Graus, J. S. Holloway, G. Huey, J. L. Jimenez, D. A. Lack, J. Liao, X. Liu, M. Z. Markovic, A. M. Middlebrook, T. Mikoviny, J. Peischl, A. E. Perring, M. S. Richardson, T. B. Ryerson, J. P. Schwarz, C. Warneke, A. Welti, A. Wisthaler, L. D. Ziemba, and D. M. Murphy
Atmos. Chem. Phys., 15, 7085–7102, https://doi.org/10.5194/acp-15-7085-2015, https://doi.org/10.5194/acp-15-7085-2015, 2015
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This paper investigates the summertime vertical profile of aerosol over the southeastern US using in situ measurements collected from aircraft. We use a vertical mixing model and measurements of CO to predict the vertical profile of aerosol that we would expect from vertical mixing alone and compare with the observed aerosol profile. We found a modest enhancement of aerosol in the cloudy transition layer during shallow cumulus convection and attribute the enhancement to local aerosol formation.
J. S. Reid, N. D. Lagrosas, H. H. Jonsson, E. A. Reid, W. R. Sessions, J. B. Simpas, S. N. Uy, T. J. Boyd, S. A. Atwood, D. R. Blake, J. R. Campbell, S. S. Cliff, B. N. Holben, R. E. Holz, E. J. Hyer, P. Lynch, S. Meinardi, D. J. Posselt, K. A. Richardson, S. V. Salinas, A. Smirnov, Q. Wang, L. Yu, and J. Zhang
Atmos. Chem. Phys., 15, 1745–1768, https://doi.org/10.5194/acp-15-1745-2015, https://doi.org/10.5194/acp-15-1745-2015, 2015
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This paper reports on the first measurements of aerosol particles embedded in the convectively active southwest monsoonal flow of the South China Sea. The paper describes the research cruise and discusses how variability in aerosol characteristics relates to regional meteorological phenomena such as and the Madden Julian Oscillation, tropical cyclones, squall lines and the monsoonal flow itself. Of special interest is how aerosol transport relates to meteorological drivers of convective activity.
C. G. Schmitt, J. D. All, J. P. Schwarz, W. P. Arnott, R. J. Cole, E. Lapham, and A. Celestian
The Cryosphere, 9, 331–340, https://doi.org/10.5194/tc-9-331-2015, https://doi.org/10.5194/tc-9-331-2015, 2015
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This paper presents the results of 3 years of measurements of light absorbing particles on the glaciers in Peru. A new analysis technique has been developed and results are shown to be well correlated with black carbon mass estimates made with the Single Particle Soot Photometer (SP2) instrument, the state-of-the-art instrument for this type of measurement. Effective black carbon levels were found to be moderate on glaciers near cities and close to zero in more remote regions.
W. R. Sessions, J. S. Reid, A. Benedetti, P. R. Colarco, A. da Silva, S. Lu, T. Sekiyama, T. Y. Tanaka, J. M. Baldasano, S. Basart, M. E. Brooks, T. F. Eck, M. Iredell, J. A. Hansen, O. C. Jorba, H.-M. H. Juang, P. Lynch, J.-J. Morcrette, S. Moorthi, J. Mulcahy, Y. Pradhan, M. Razinger, C. B. Sampson, J. Wang, and D. L. Westphal
Atmos. Chem. Phys., 15, 335–362, https://doi.org/10.5194/acp-15-335-2015, https://doi.org/10.5194/acp-15-335-2015, 2015
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B. H. Samset, G. Myhre, A. Herber, Y. Kondo, S.-M. Li, N. Moteki, M. Koike, N. Oshima, J. P. Schwarz, Y. Balkanski, S. E. Bauer, N. Bellouin, T. K. Berntsen, H. Bian, M. Chin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, M. Schulz, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 14, 12465–12477, https://doi.org/10.5194/acp-14-12465-2014, https://doi.org/10.5194/acp-14-12465-2014, 2014
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Far from black carbon (BC) emission sources, present climate models are unable to reproduce flight measurements. By comparing recent models with data, we find that the atmospheric lifetime of BC may be overestimated in models. By adjusting modeled BC concentrations to measurements in remote regions - over oceans and at high altitudes - we arrive at a reduced estimate for BC radiative forcing over the industrial era.
X. Wang, C. L. Heald, D. A. Ridley, J. P. Schwarz, J. R. Spackman, A. E. Perring, H. Coe, D. Liu, and A. D. Clarke
Atmos. Chem. Phys., 14, 10989–11010, https://doi.org/10.5194/acp-14-10989-2014, https://doi.org/10.5194/acp-14-10989-2014, 2014
S. S. Brown, W. P. Dubé, R. Bahreini, A. M. Middlebrook, C. A. Brock, C. Warneke, J. A. de Gouw, R. A. Washenfelder, E. Atlas, J. Peischl, T. B. Ryerson, J. S. Holloway, J. P. Schwarz, R. Spackman, M. Trainer, D. D. Parrish, F. C. Fehshenfeld, and A. R. Ravishankara
Atmos. Chem. Phys., 13, 11317–11337, https://doi.org/10.5194/acp-13-11317-2013, https://doi.org/10.5194/acp-13-11317-2013, 2013
Z. Kipling, P. Stier, J. P. Schwarz, A. E. Perring, J. R. Spackman, G. W. Mann, C. E. Johnson, and P. J. Telford
Atmos. Chem. Phys., 13, 5969–5986, https://doi.org/10.5194/acp-13-5969-2013, https://doi.org/10.5194/acp-13-5969-2013, 2013
M. Laborde, M. Schnaiter, C. Linke, H. Saathoff, K.-H. Naumann, O. Möhler, S. Berlenz, U. Wagner, J. W. Taylor, D. Liu, M. Flynn, J. D. Allan, H. Coe, K. Heimerl, F. Dahlkötter, B. Weinzierl, A. G. Wollny, M. Zanatta, J. Cozic, P. Laj, R. Hitzenberger, J. P. Schwarz, and M. Gysel
Atmos. Meas. Tech., 5, 3077–3097, https://doi.org/10.5194/amt-5-3077-2012, https://doi.org/10.5194/amt-5-3077-2012, 2012
Related subject area
Discipline: Snow | Subject: Atmospheric Interactions
Identifying airborne snow metamorphism with stable water isotopes
Seasonal snow–atmosphere modeling: let's do it
On the importance to consider the cloud dependence in parameterizing the albedo of snow on sea ice
Understanding snow saltation parameterizations: lessons from theory, experiments and numerical simulations
A novel framework to investigate wind-driven snow redistribution over an Alpine glacier: combination of high-resolution terrestrial laser scans and large-eddy simulations
From atmospheric water isotopes measurement to firn core interpretation in Adélie Land: a case study for isotope-enabled atmospheric models in Antarctica
Dynamics of the snow grain size in a windy coastal area of Antarctica from continuous in situ spectral-albedo measurements
Forcing and impact of the Northern Hemisphere continental snow cover in 1979–2014
On the energy budget of a low-Arctic snowpack
The role of sublimation as a driver of climate signals in the water isotope content of surface snow: laboratory and field experimental results
Synoptic control on snow avalanche activity in central Spitsbergen
Interfacial supercooling and the precipitation of hydrohalite in frozen NaCl solutions as seen by X-ray absorption spectroscopy
Tracing devastating fires in Portugal to a snow archive in the Swiss Alps: a case study
Systematic bias of Tibetan Plateau snow cover in subseasonal-to-seasonal models
Warm-air entrainment and advection during alpine blowing snow events
Quantifying the impact of synoptic weather types and patterns on energy fluxes of a marginal snowpack
Radar measurements of blowing snow off a mountain ridge
Brief communication: Rare ambient saturation during drifting snow occurrences at a coastal location of East Antarctica
Understanding snow bedform formation by adding sintering to a cellular automata model
Evaluation of snow depth and snow cover over the Tibetan Plateau in global reanalyses using in situ and satellite remote sensing observations
Brief communication: Analysis of organic matter in surface snow by PTR-MS – implications for dry deposition dynamics in the Alps
Evaluation of the CloudSat surface snowfall product over Antarctica using ground-based precipitation radars
Sonja Wahl, Benjamin Walter, Franziska Aemisegger, Luca Bianchi, and Michael Lehning
The Cryosphere, 18, 4493–4515, https://doi.org/10.5194/tc-18-4493-2024, https://doi.org/10.5194/tc-18-4493-2024, 2024
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Wind-driven airborne transport of snow is a frequent phenomenon in snow-covered regions and a process difficult to study in the field as it is unfolding over large distances. Thus, we use a ring wind tunnel with infinite fetch positioned in a cold laboratory to study the evolution of the shape and size of airborne snow. With the help of stable water isotope analyses, we identify the hitherto unobserved process of airborne snow metamorphism that leads to snow particle rounding and growth.
Dylan Reynolds, Louis Quéno, Michael Lehning, Mahdi Jafari, Justine Berg, Tobias Jonas, Michael Haugeneder, and Rebecca Mott
The Cryosphere, 18, 4315–4333, https://doi.org/10.5194/tc-18-4315-2024, https://doi.org/10.5194/tc-18-4315-2024, 2024
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Information about atmospheric variables is needed to produce simulations of mountain snowpacks. We present a model that can represent processes that shape mountain snowpack, focusing on the accumulation of snow. Simulations show that this model can simulate the complex path that a snowflake takes towards the ground and that this leads to differences in the distribution of snow by the end of winter. Overall, this model shows promise with regard to improving forecasts of snow in mountains.
Lara Foth, Wolfgang Dorn, Annette Rinke, Evelyn Jäkel, and Hannah Niehaus
The Cryosphere, 18, 4053–4064, https://doi.org/10.5194/tc-18-4053-2024, https://doi.org/10.5194/tc-18-4053-2024, 2024
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It is demonstrated that the explicit consideration of the cloud dependence of the snow surface albedo in a climate model results in a more realistic simulation of the surface albedo during the snowmelt period in late May and June. Although this improvement appears to be relatively insubstantial, it has significant impact on the simulated sea-ice volume and extent in the model due to an amplification of the snow/sea-ice albedo feedback, one of the main contributors to Arctic amplification.
Daniela Brito Melo, Armin Sigmund, and Michael Lehning
The Cryosphere, 18, 1287–1313, https://doi.org/10.5194/tc-18-1287-2024, https://doi.org/10.5194/tc-18-1287-2024, 2024
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Snow saltation – the transport of snow close to the surface – occurs when the wind blows over a snow-covered surface with sufficient strength. This phenomenon is represented in some climate models; however, with limited accuracy. By performing numerical simulations and a detailed analysis of previous works, we show that snow saltation is characterized by two regimes. This is not represented in climate models in a consistent way, which hinders the quantification of snow transport and sublimation.
Annelies Voordendag, Brigitta Goger, Rainer Prinz, Tobias Sauter, Thomas Mölg, Manuel Saigger, and Georg Kaser
The Cryosphere, 18, 849–868, https://doi.org/10.5194/tc-18-849-2024, https://doi.org/10.5194/tc-18-849-2024, 2024
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Wind-driven snow redistribution affects glacier mass balance. A case study of Hintereisferner glacier in Austria used high-resolution observations and simulations to model snow redistribution. Simulations matched observations, showing the potential of the model for studying snow redistribution on other mountain glaciers.
Christophe Leroy-Dos Santos, Elise Fourré, Cécile Agosta, Mathieu Casado, Alexandre Cauquoin, Martin Werner, Benedicte Minster, Frédéric Prié, Olivier Jossoud, Leila Petit, and Amaëlle Landais
The Cryosphere, 17, 5241–5254, https://doi.org/10.5194/tc-17-5241-2023, https://doi.org/10.5194/tc-17-5241-2023, 2023
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In the face of global warming, understanding the changing water cycle and temperatures in polar regions is crucial. These factors directly impact the balance of ice sheets in the Arctic and Antarctic. By studying the composition of water vapor, we gain insights into climate variations. Our 2-year study at Dumont d’Urville station, Adélie Land, offers valuable data to refine models. Additionally, we demonstrate how modeling aids in interpreting signals from ice core samples in the region.
Sara Arioli, Ghislain Picard, Laurent Arnaud, and Vincent Favier
The Cryosphere, 17, 2323–2342, https://doi.org/10.5194/tc-17-2323-2023, https://doi.org/10.5194/tc-17-2323-2023, 2023
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To assess the drivers of the snow grain size evolution during snow drift, we exploit a 5-year time series of the snow grain size retrieved from spectral-albedo observations made with a new, autonomous, multi-band radiometer and compare it to observations of snow drift, snowfall and snowmelt at a windy location of coastal Antarctica. Our results highlight the complexity of the grain size evolution in the presence of snow drift and show an overall tendency of snow drift to limit its variations.
Guillaume Gastineau, Claude Frankignoul, Yongqi Gao, Yu-Chiao Liang, Young-Oh Kwon, Annalisa Cherchi, Rohit Ghosh, Elisa Manzini, Daniela Matei, Jennifer Mecking, Lingling Suo, Tian Tian, Shuting Yang, and Ying Zhang
The Cryosphere, 17, 2157–2184, https://doi.org/10.5194/tc-17-2157-2023, https://doi.org/10.5194/tc-17-2157-2023, 2023
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Snow cover variability is important for many human activities. This study aims to understand the main drivers of snow cover in observations and models in order to better understand it and guide the improvement of climate models and forecasting systems. Analyses reveal a dominant role for sea surface temperature in the Pacific. Winter snow cover is also found to have important two-way interactions with the troposphere and stratosphere. No robust influence of the sea ice concentration is found.
Georg Lackner, Florent Domine, Daniel F. Nadeau, Annie-Claude Parent, François Anctil, Matthieu Lafaysse, and Marie Dumont
The Cryosphere, 16, 127–142, https://doi.org/10.5194/tc-16-127-2022, https://doi.org/10.5194/tc-16-127-2022, 2022
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The surface energy budget is the sum of all incoming and outgoing energy fluxes at the Earth's surface and has a key role in the climate. We measured all these fluxes for an Arctic snowpack and found that most incoming energy from radiation is counterbalanced by thermal radiation and heat convection while sublimation was negligible. Overall, the snow model Crocus was able to simulate the observed energy fluxes well.
Abigail G. Hughes, Sonja Wahl, Tyler R. Jones, Alexandra Zuhr, Maria Hörhold, James W. C. White, and Hans Christian Steen-Larsen
The Cryosphere, 15, 4949–4974, https://doi.org/10.5194/tc-15-4949-2021, https://doi.org/10.5194/tc-15-4949-2021, 2021
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Water isotope records in Greenland and Antarctic ice cores are a valuable proxy for paleoclimate reconstruction and are traditionally thought to primarily reflect precipitation input. However,
post-depositional processes are hypothesized to contribute to the isotope climate signal. In this study we use laboratory experiments, field experiments, and modeling to show that sublimation and vapor–snow isotope exchange can rapidly influence the isotopic composition of the snowpack.
Holt Hancock, Jordy Hendrikx, Markus Eckerstorfer, and Siiri Wickström
The Cryosphere, 15, 3813–3837, https://doi.org/10.5194/tc-15-3813-2021, https://doi.org/10.5194/tc-15-3813-2021, 2021
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We investigate how snow avalanche activity in central Spitsbergen, Svalbard, is broadly controlled by atmospheric circulation. Avalanche activity in this region is generally associated with atmospheric circulation conducive to increased precipitation, wind speeds, and air temperatures near Svalbard during winter storms. Our results help place avalanche activity on Spitsbergen in the wider context of Arctic environmental change and provide a foundation for improved avalanche forecasting here.
Thorsten Bartels-Rausch, Xiangrui Kong, Fabrizio Orlando, Luca Artiglia, Astrid Waldner, Thomas Huthwelker, and Markus Ammann
The Cryosphere, 15, 2001–2020, https://doi.org/10.5194/tc-15-2001-2021, https://doi.org/10.5194/tc-15-2001-2021, 2021
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Chemical reactions in sea salt embedded in coastal polar snow impact the composition and air quality of the atmosphere. Here, we investigate the phase changes of sodium chloride. This is of importance as chemical reactions proceed faster in liquid solutions compared to in solid salt and the precise precipitation temperature of sodium chloride is still under debate. We focus on the upper nanometres of sodium chloride–ice samples because of their role as a reactive interface in the environment.
Dimitri Osmont, Sandra Brugger, Anina Gilgen, Helga Weber, Michael Sigl, Robin L. Modini, Christoph Schwörer, Willy Tinner, Stefan Wunderle, and Margit Schwikowski
The Cryosphere, 14, 3731–3745, https://doi.org/10.5194/tc-14-3731-2020, https://doi.org/10.5194/tc-14-3731-2020, 2020
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In this interdisciplinary case study, we were able to link biomass burning emissions from the June 2017 wildfires in Portugal to their deposition in the snowpack at Jungfraujoch, Swiss Alps. We analysed black carbon and charcoal in the snowpack, calculated backward trajectories, and monitored the fire evolution by remote sensing. Such case studies help to understand the representativity of biomass burning records in ice cores and how biomass burning tracers are archived in the snowpack.
Wenkai Li, Shuzhen Hu, Pang-Chi Hsu, Weidong Guo, and Jiangfeng Wei
The Cryosphere, 14, 3565–3579, https://doi.org/10.5194/tc-14-3565-2020, https://doi.org/10.5194/tc-14-3565-2020, 2020
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Understanding the forecasting skills of the subseasonal-to-seasonal (S2S) model on Tibetan Plateau snow cover (TPSC) is the first step to applying the S2S model to hydrological forecasts over the Tibetan Plateau. This study conducted a multimodel comparison of the TPSC prediction skill to learn about their performance in capturing TPSC variability. S2S models can skillfully forecast TPSC within a lead time of 2 weeks but show limited skill beyond 3 weeks. Systematic biases of TPSC were found.
Nikolas O. Aksamit and John W. Pomeroy
The Cryosphere, 14, 2795–2807, https://doi.org/10.5194/tc-14-2795-2020, https://doi.org/10.5194/tc-14-2795-2020, 2020
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In cold regions, it is increasingly important to quantify the amount of water stored as snow at the end of winter. Current models are inconsistent in their estimates of snow sublimation due to atmospheric turbulence. Specific wind structures have been identified that amplify potential rates of surface and blowing snow sublimation during blowing snow storms. The recurrence of these motions has been modeled by a simple scaling argument that has its foundation in turbulent boundary layer theory.
Andrew J. Schwartz, Hamish A. McGowan, Alison Theobald, and Nik Callow
The Cryosphere, 14, 2755–2774, https://doi.org/10.5194/tc-14-2755-2020, https://doi.org/10.5194/tc-14-2755-2020, 2020
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This study measured energy available for snowmelt during the 2016 and 2017 snow seasons in Kosciuszko National Park, NSW, Australia, and identified common traits for days with similar weather characteristics. The analysis showed that energy available for snowmelt was highest in the days before cold fronts passed through the region due to higher air temperatures. Regardless of differences in daily weather characteristics, solar radiation contributed the highest amount of energy to snowpack melt.
Benjamin Walter, Hendrik Huwald, Josué Gehring, Yves Bühler, and Michael Lehning
The Cryosphere, 14, 1779–1794, https://doi.org/10.5194/tc-14-1779-2020, https://doi.org/10.5194/tc-14-1779-2020, 2020
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We applied a horizontally mounted low-cost precipitation radar to measure velocities, frequency of occurrence, travel distances and turbulence characteristics of blowing snow off a mountain ridge. Our analysis provides a first insight into the potential of radar measurements for determining blowing snow characteristics, improves our understanding of mountain ridge blowing snow events and serves as a valuable data basis for validating coupled numerical weather and snowpack simulations.
Charles Amory and Christoph Kittel
The Cryosphere, 13, 3405–3412, https://doi.org/10.5194/tc-13-3405-2019, https://doi.org/10.5194/tc-13-3405-2019, 2019
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Snow mass fluxes and vertical profiles of relative humidity are used to document concurrent occurrences of drifting snow and near-surface air saturation at a site dominated by katabatic winds in East Antarctica. Despite a high prevalence of drifting snow conditions, we demonstrate that saturation is reached only in the most extreme wind and transport conditions and discuss implications for the understanding of surface mass and atmospheric moisture budgets of the Antarctic ice sheet.
Varun Sharma, Louise Braud, and Michael Lehning
The Cryosphere, 13, 3239–3260, https://doi.org/10.5194/tc-13-3239-2019, https://doi.org/10.5194/tc-13-3239-2019, 2019
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Snow surfaces, under the action of wind, form beautiful shapes such as waves and dunes. This study is the first ever study to simulate these shapes using a state-of-the-art numerical modelling tool. While these beautiful and ephemeral shapes on snow surfaces are fascinating from a purely aesthetic point of view, they are also critical in regulating the transfer of heat and mass between the atmosphere and snowpacks, thus being of huge importance to the Earth system.
Yvan Orsolini, Martin Wegmann, Emanuel Dutra, Boqi Liu, Gianpaolo Balsamo, Kun Yang, Patricia de Rosnay, Congwen Zhu, Wenli Wang, Retish Senan, and Gabriele Arduini
The Cryosphere, 13, 2221–2239, https://doi.org/10.5194/tc-13-2221-2019, https://doi.org/10.5194/tc-13-2221-2019, 2019
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The Tibetan Plateau region exerts a considerable influence on regional climate, yet the snowpack over that region is poorly represented in both climate and forecast models due a large precipitation and snowfall bias. We evaluate the snowpack in state-of-the-art atmospheric reanalyses against in situ observations and satellite remote sensing products. Improved snow initialisation through better use of snow observations in reanalyses may improve medium-range to seasonal weather forecasts.
Dušan Materić, Elke Ludewig, Kangming Xu, Thomas Röckmann, and Rupert Holzinger
The Cryosphere, 13, 297–307, https://doi.org/10.5194/tc-13-297-2019, https://doi.org/10.5194/tc-13-297-2019, 2019
Niels Souverijns, Alexandra Gossart, Stef Lhermitte, Irina V. Gorodetskaya, Jacopo Grazioli, Alexis Berne, Claudio Duran-Alarcon, Brice Boudevillain, Christophe Genthon, Claudio Scarchilli, and Nicole P. M. van Lipzig
The Cryosphere, 12, 3775–3789, https://doi.org/10.5194/tc-12-3775-2018, https://doi.org/10.5194/tc-12-3775-2018, 2018
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Snowfall observations over Antarctica are scarce and currently limited to information from the CloudSat satellite. Here, a first evaluation of the CloudSat snowfall record is performed using observations of ground-based precipitation radars. Results indicate an accurate representation of the snowfall climatology over Antarctica, despite the low overpass frequency of the satellite, outperforming state-of-the-art model estimates. Individual snowfall events are however not well represented.
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Short summary
Ice–albedo feedbacks in the ablation region of the Greenland Ice Sheet are difficult to constrain and model. Surface samples were collected across the 2014 summer melt season from different ice surface colors. On average, concentrations were higher in patches that were visibly dark, compared to medium patches and light patches, suggesting that black carbon aggregation contributed to snow aging, and vice versa. High concentrations are likely due to smoke transport from high-latitude wildfires.
Ice–albedo feedbacks in the ablation region of the Greenland Ice Sheet are difficult to...